Effect of Different Gypsum Particle Morphologies on the Properties of Lightweight Polyethylene/Fly Ash/Gypsum Composite
Abstract
In recent years, the development of sustainable materials from industrial mineral wastes or by-products have gained importance to achieve carbon neutrality. Among these industrial wastes, fly ash (FA) and flue gas desulfurization (FGD) gypsum are two significant by-products generated in large quantities by coal-fired thermal power stations, and their valorization has become a critical research topic. This study focuses on the development of composite materials using fly ash and FGD gypsum in combination, with low-density polyethylene (PE) as the binder. In addition, borogypsum (BG), which has a higher particle aspect ratio than FGD gypsum, was also used instead of FGD gypsum, and changes in the composite properties were evaluated. With the addition of borogypsum, 32.8% higher strength values were obtained compared to the series containing FGD gypsum. The results indicate that composite structures incorporating both phases yield a more balanced microstructure and enhanced mechanical performance compared to those in which UK, FGD, or BG is used individually. Additionally, SEM images illustrate the elongation and breakage of the PE binder matrix during fracture, confirming its dominant role in strength development. It was concluded that particle morphologies and loose particle density of the different gypsum filler materials in lightweight Polyethylene/Fly Ash/Gypsum composites are important factors. It should also be noted that the particle size distributions of two different gypsums were also effective in determining the physical-mechanical properties.
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References
- 1. Muthukutti, G. P., Singh, M. K., Palaniappan, S. K., Vijayananth, K., Rangappa, S. M., & Siengchin, S. (2025). Value-added polymer composites using non-metallic industrial waste: A concise review. Chemical Engineering Journal, 162344. https://doi.org/10.1016/j.cej.2025.162344
- 2. Li, Z., Li, W., You, J., Huang, J., Gan, R., Guo, J., & Zhang, X. (2024). Critical secondary resource for porous ceramics: A review on recycling of inorganic solid wastes. Journal of the European Ceramic Society, 44(15), 116781. https://doi.org/10.1016/j.jeurceramsoc.2024.116781
- 3. Wang, M., Chen, D., Wang, H., & Gao, W. (2024). A review on fly ash high-value synthesis utilization and its prospect. Green Energy and Resources, 2(1), 100062. https://doi.org/10.1016/j.gerr.2024.100062
- 4. Hawileh, R. A., Shaw, S. K., Assad, M., Dey, A., Abdalla, J. A., & Kim, J. H. (2025). Influence of Fly Ash on the Compressive Strength of Ultrahigh-Performance Concrete: A State-of-the-art Review To-wards Sustainability. International Journal of Concrete Structures and Materials, 19(1), 1-28. https://doi.org/10.1186/s40069-024-00757-x
- 5. Alterary, S. S., & Marei, N. H. (2021). Fly ash properties, characteri-zation, and applications: A review. Journal of King Saud University-Science, 33(6), 101536. https://doi.org/10.1016/j.jksus.2021.101536
- 6. Kuźnia, M. (2024). A review of coal fly Ash utilization: environmen-tal, energy, and material assessment. Energies, 18(1), 52. https://doi.org/10.3390/en18010052
- 7. Ram, A. K., & Mohanty, S. (2022). State of the art review on physio-chemical and engineering characteristics of fly ash and its applica-tions. International Journal of Coal Science & Technology, 9(1), 9. https://doi.org/10.1007/s40789-022-00472-6
- 8. Ninteretse, J. D. D., Nshimiyimana, M., Niyogisubizo, J., Sugira, J. C., & Niyongabo, A. (2024). Assessing Mechanical Properties of Free-Fall Self-Compacting Concrete and its Application in Concrete-Filled Steel Tube Columns. Engineering Perspective, 4(2), 84-94. https://doi.org/10.29228/eng.pers.76064
Details
Primary Language
English
Subjects
Environmental and Sustainable Processes, Materials Science and Technologies, Polymer Science and Technologies, Composite and Hybrid Materials, Material Characterization
Journal Section
Research Article
Publication Date
February 24, 2026
Submission Date
December 12, 2025
Acceptance Date
February 20, 2026
Published in Issue
Year 2026 Volume: 6 Number: 1
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