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Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites

Year 2024, Volume: 13 Issue: 3, 232 - 248, 31.12.2024
https://doi.org/10.54187/jnrs.1569548

Abstract

In this comprehensive study, we meticulously fabricated Al-30Sm2O3-XGd2O3 (X = 3, 6, 9, 12, and 15) composites through a series of tests and analyses to determine the composites' mechanical, physical, corrosion, and radiation shielding properties. Scanning electron microscopy (SEM-EDX) and X-ray diffraction (XRD) techniques were used for microstructural analysis. The main objective of the research is to investigate the effects of Gd2O3 reinforcement on the mechanical properties (hardness, wear resistance, and corrosion resistance) and radiation shielding performances of the composites. MCNP6.2 simulations evaluated thermal, fast neutron, and gamma-ray attenuation properties, while mechanical properties were analyzed by hardness, wear, and corrosion tests. XRD analyses showed no intermetallic phase was formed, while SEM-EDX analyses revealed that the composites were homogeneous and had a partial increase in void ratio with Gd2O3 reinforcement. Gd2O3 reinforcement increased the hardness and wear resistance of the composites, but a slight decrease in relative density was observed. The highest hardness and wear resistance were obtained at 15% Gd2O3 reinforcement. The corrosion rate decreased with Gd2O3 reinforcement, while an increase in corrosion rate was observed in the composite containing 15% Gd2O3. MCNP6.2 simulations showed that Gd2O3 reinforcement increased the thermal neutron macroscopic cross-section and linear attenuation coefficient while decreasing the fast neutron macroscopic cross-section.

References

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  • P. Zhang, C. Jia, J. Li, W. Wang, Shielding composites for neutron and gamma-radiation with Gd2O3@W core-shell structured particles, Materials Letters 276 (2020) 128082.
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  • M. C. Team, MCNP-A general Monte Carlo N-particle transport code, Version 5 Volume I: Overview and Theory X-5 Monte Carlo Team, 2003.
  • H. Ozdogan, O. Kilicoglu, F. Akman, O. Agar, Comparison of Monte Carlo simulations and theoretical calculations of nuclear shielding characteristics of various borate glasses including Bi, V, Fe, and Cd, Applied Radiation and Isotopes 189 (2022) 110454.
  • S. Caglar, M. F. Kilicaslan, A. Atasoy, H. Tiryaki, M. Erkovan, S. jik Hong, Effect of heat treatment on magnetic properties of nanocomposite Nd-lean Nd7Fe73B20 ribbons, Journal of Materials Science: Materials in Electronics 32 (2021) 2338–2345.
  • Y. Zhu, T. Zhao, X. Yu, Y. Zhu, Q. Shen, R. Li, G. Xie, Effect of gadolinium trioxide on anode performance of aluminum-air batteries, Ionics 29 (2023) 4723–4731.
  • H. Akyıldırım, Calculation of fast neutron shielding parameters for some essential carbohydrates, Erzincan University Journal of Science and Technology 12 (2019) 1141–1148.
Year 2024, Volume: 13 Issue: 3, 232 - 248, 31.12.2024
https://doi.org/10.54187/jnrs.1569548

Abstract

References

  • M. Lalkovicova, Neuroprotective agents effective against radiation damage of central nervous system, Neural Regeneration Research 17 (2022) 1885–1892.
  • G.A. Thomas, P. Symonds, Radiation Exposure and Health Effects - is it Time to Reassess the Real Consequences?. Clinical Oncology, (2016) 28(4), 231–236.
  • Y. Gaylan, B. Avar, Al–B4C-(Gd, Gd2O3) composite materials: Synthesis and characterization for neutron shielding applications, Nuclear Engineering and Technology (2024).
  • N. Ekinci, N.A.M. Alsaif, Z.Y. Khattari, Y.S. Rammah, B. Aygün, Y. Kurucu, S. Sarıtaş, Evaluation of lithium tetra borate glass-ceramics: Structural, physical and radiation safety properties using experimental and theoretical methods, Nuclear Engineering and Technology (2024).
  • B. Aygun, I. Bilici, C.U. Deniz, B. Oz, M.I. Sayyed, A. Karabulut, Development of novel composite materials containing rice bran wax and waste polyethylene for neutron shielding applications, Progress in Nuclear Energy 174 (2024) 105262.
  • C. Kursun, M. Gao, S. Guclu, Y. Gaylan, K.A. Parrey, A.O. Yalcin, Measurement on the neutron and gamma radiation shielding performance of boron-doped titanium alloy Ti 50 Cu 30 Zr 15 B 5 via arc melting technique, Heliyon 9 (2023) 2405–8440.
  • H.S. Chen, W.X. Wang, Y.L. Li, P. Zhang, H.H. Nie, Q.C. Wu, M. Carlo, The design, microstructure and tensile properties of B4C particulate reinforced 6061Al neutron absorber composites, Journal of Alloys and Compounds 632 (2015) 23–29.
  • K. Deng, J. Shi, C. Wang, X. Wang, Y. Wu, K. Nie, K. Wu, Composites: Part A Microstructure and strengthening mechanism of bimodal size particle reinforced magnesium matrix composite, Composites Part A 43 (2012) 1280–1284.
  • G. Luo, J. Wu, S. Xiong, Q. Shen, C. Wu, Microstructure and mechanical behavior of AA2024 / B 4 C composites with a network reinforcement architecture, Journal of Alloys and Compounds 701 (2017) 554–561.
  • I. Topcu, H. O. Gulsoy, N. Kadioglu, A. N. Gulluoglu, Processing and mechanical properties of B4C reinforced Al matrix composites, Journal of Alloys and Compounds 482 (2009) 516–521.
  • P. Zhang, Y. Li, W. Wang, Z. Gao, B. Wang, The design, fabrication and properties of B4C/Al neutron absorbers, Journal of Nuclear Materials 437 (2013) 350–358.
  • Y. Gaylan, B. Avar, M. Panigrahi, B. Aygün, A. Karabulut, Effect of the B4C content on microstructure, microhardness, corrosion, and neutron shielding properties of Al–B4C composites, Ceramics International 49 (2023) 5479–5488.
  • Y. He, H. Xu, Y. Liu, Y. Chen, Z. Ji, Strengthening mechanism of B4C@APC/Al matrix composites reinforced with bimodal-sized particles prepared by hydrothermal carbonized deposition on chips, Journal of Materials Science & Technology 123 (2022) 60–69.
  • R. G. Abrefah, R. B. M. Sogbadji, E. Ampomah-Amoako, S. A. Birikorang, H. C. Odoi, B. J. B. Nyarko, Comparison of the effects of cadmium-shielded and boron carbide-shielded irradiation channel of the Ghana Research Reactor-1, Nuclear Engineering and Design 241 (2011) 3017–3020.
  • S. Wan, W. Wang, H. Chen, J. Zhou, Y. Zhang, R. Liu, R. Feng, 155/157Gd areal density: A model for design and fabrication of Gd2O3/316L novel neutron shielding composites, Vacuum 176 (2020).
  • R. Florez, H. A. Colorado, C. H. C. Giraldo, A. Alajo, Preparation and characterization of Portland cement pastes with Sm2O3 microparticle additions for neutron shielding applications, Construction and Building Materials 191 (2018) 498–506.
  • C. Kursun, M. Gao, A. O. Yalcin, K. A. Parrey, Y. Gaylan, Structure, mechanical, and neutron radiation shielding characteristics of mechanically milled nanostructured (100-x)Al-xGd2O3 metal composites, Ceramics International (2024).
  • D.-Y. Zhang, X.-Y. Shen, Q. Ruan, X.-L. Xu, S.-P. Yang, Y. Lu, H.-Y. Xu, F.-L. Hao, Effects of subchronic samarium exposure on the histopathological structure and apoptosis regulation in mouse testis, Environ Toxicol Pharmacol 37 (2014) 505–512.
  • Y. Gaylan, I. E. Dag, S. Caglar, B. Avar, Investigation of mechanical and radiation shielding properties of Sm–Sm2O3 reinforced Al–B4C composite, Radiation Physics and Chemistry 226 (2025) 112325.
  • H. Guo, Z. Zhang, Y. Zhang, Y. Cui, L. Sun, D. Chen, Improving the mechanical properties of B4C/Al composites by solid-state interfacial reaction, Journal of Alloys and Compounds 829 (2020) 154521.
  • Q. Lin, P. Shen, F. Qiu, D. Zhang, Q. Jiang, Wetting of polycrystalline B4C by molten Al at 1173–1473K, Scripta Materialia 60 (2009) 960–963.
  • R.-F. Guo, S.-M. Chen, P. Shen, Influence of Si, Ti, and Cu as alloying elements on the wettability and reactivity of an Al/B4C system, Journal of Materials Research and Technology 27 (2023) 6104–6116.
  • L. T. Jiang, Z. G. Xu, Y. K. Fei, Q. Zhang, J. Qiao, G. H. Wu, The design of novel neutron shielding (Gd+B4C)/6061Al composites and its properties after hot rolling, Composites Part B: Engineering 168 (2019) 183–194.
  • P. Zhang, C. Jia, J. Li, W. Wang, Shielding composites for neutron and gamma-radiation with Gd2O3@W core-shell structured particles, Materials Letters 276 (2020) 128082.
  • S. Niksarlıoğlu, F. Akman, M.E. Pekdemir, S. Yalçın Kuzu, M.R. Kaçal, M. Yılmaz, An extensive investigation on gamma shielding properties of PLA/Gd2O3 nanocomposites, Radiation Physics and Chemistry 208 (2023) 110936.
  • S. Cong, Y. Li, G. Ran, W. Zhou, Q. Feng, Microstructure and its effect on mechanical and thermal properties of Al-based Gd2O3 MMCs used as shielding materials in spent fuel storage, Ceramics International 46 (2020) 12986–12995.
  • M. C. Team, MCNP-A general Monte Carlo N-particle transport code, Version 5 Volume I: Overview and Theory X-5 Monte Carlo Team, 2003.
  • H. Ozdogan, O. Kilicoglu, F. Akman, O. Agar, Comparison of Monte Carlo simulations and theoretical calculations of nuclear shielding characteristics of various borate glasses including Bi, V, Fe, and Cd, Applied Radiation and Isotopes 189 (2022) 110454.
  • S. Caglar, M. F. Kilicaslan, A. Atasoy, H. Tiryaki, M. Erkovan, S. jik Hong, Effect of heat treatment on magnetic properties of nanocomposite Nd-lean Nd7Fe73B20 ribbons, Journal of Materials Science: Materials in Electronics 32 (2021) 2338–2345.
  • Y. Zhu, T. Zhao, X. Yu, Y. Zhu, Q. Shen, R. Li, G. Xie, Effect of gadolinium trioxide on anode performance of aluminum-air batteries, Ionics 29 (2023) 4723–4731.
  • H. Akyıldırım, Calculation of fast neutron shielding parameters for some essential carbohydrates, Erzincan University Journal of Science and Technology 12 (2019) 1141–1148.
There are 31 citations in total.

Details

Primary Language English
Subjects Material Physics, Nuclear Physics
Journal Section Articles
Authors

Seyit Çağlar 0000-0002-0701-3029

Publication Date December 31, 2024
Submission Date October 18, 2024
Acceptance Date December 20, 2024
Published in Issue Year 2024 Volume: 13 Issue: 3

Cite

APA Çağlar, S. (2024). Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites. Journal of New Results in Science, 13(3), 232-248. https://doi.org/10.54187/jnrs.1569548
AMA Çağlar S. Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites. JNRS. December 2024;13(3):232-248. doi:10.54187/jnrs.1569548
Chicago Çağlar, Seyit. “Influence of Gd2O3 Reinforcement on the Mechanical, Physical and Radiation Shielding Properties of Al-30Sm2O3 Composites”. Journal of New Results in Science 13, no. 3 (December 2024): 232-48. https://doi.org/10.54187/jnrs.1569548.
EndNote Çağlar S (December 1, 2024) Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites. Journal of New Results in Science 13 3 232–248.
IEEE S. Çağlar, “Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites”, JNRS, vol. 13, no. 3, pp. 232–248, 2024, doi: 10.54187/jnrs.1569548.
ISNAD Çağlar, Seyit. “Influence of Gd2O3 Reinforcement on the Mechanical, Physical and Radiation Shielding Properties of Al-30Sm2O3 Composites”. Journal of New Results in Science 13/3 (December 2024), 232-248. https://doi.org/10.54187/jnrs.1569548.
JAMA Çağlar S. Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites. JNRS. 2024;13:232–248.
MLA Çağlar, Seyit. “Influence of Gd2O3 Reinforcement on the Mechanical, Physical and Radiation Shielding Properties of Al-30Sm2O3 Composites”. Journal of New Results in Science, vol. 13, no. 3, 2024, pp. 232-48, doi:10.54187/jnrs.1569548.
Vancouver Çağlar S. Influence of Gd2O3 reinforcement on the mechanical, physical and radiation shielding properties of Al-30Sm2O3 composites. JNRS. 2024;13(3):232-48.


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