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Year 2020, Volume: 38 Issue: 4, 1791 - 1810, 05.10.2021

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References

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ENERGY CONSUMPTION AND EFFICIENCY IMPROVEMENT OF ELECTRO-ACTIVATED PERSULFATE PROCESSES: OPTIMIZATION BY CCD FOR TOC REMOVAL FROM LEACHATE CONCENTRATE

Year 2020, Volume: 38 Issue: 4, 1791 - 1810, 05.10.2021

Abstract

This study aimed to investigate the application of electro-activated persulfate processes to provide maximum total organic carbon (TOC) removal from the leachate nanofiltration concentrate with minimum energy consumption. Electro-activated persulfate processes were evaluated in terms of operating parameters of oxidant/chemical oxygen demand (COD) ratio, applied current, pH, and reaction time. Response surface methodology and central composite design were applied for statistical analysis and optimization of process parameters. Estimated TOC removal efficiencies by the model under optimum conditions were 58.65% and 61.07% for electro-peroxymonosulfate (EPM) and electro-peroxydisulfate (EPD) processes, respectively; while energy consumption was 1.87 and 5.81 kWh/m3, respectively. TOC removal efficiencies in experimental studies performed to verify model conformity were 56.91% and 58.43% for EPM and EPD processes, respectively. The conformity of the estimated and actual removal efficiencies shows that the central composite design is a suitable tool in determining the optimum conditions to achieve maximum TOC removal with minimum cost. Since the TOC removal efficiencies obtained by EPM and EPD processes were very close to each other, the EPM process with lower energy consumption is more advantageous.
Based on the experimental results, a mathematical model was developed, and the nickel inhibition constants (KNi) were found to be 8.75 mg/L.

References

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  • ⦁ Antony, J., Niveditha, S. V., Gandhimathi, R., Ramesh, S.T., Nidheesh, P. V., 2020. Stabilized landfill leachate treatment by zero valent aluminium-acid system combined with hydrogen peroxide and persulfate based advanced oxidation process. Waste Manag. 106, 1–11. https://doi.org/10.1016/j.wasman.2020.03.005
  • ⦁ APHA, 2005. Standard Methods for Examination of Water and Wastewater, 21th ed, American Public Health Association. American Public Health Association. https://doi.org/ISBN 9780875532356
  • ⦁ Arslan-Alaton, I., Olmez-Hanci, T., Khoei, S., Fakhri, H., 2017. Oxidative degradation of Triton X-45 using zero valent aluminum in the presence of hydrogen peroxide, persulfate and peroxymonosulfate. Catal. Today 280, 199–207. https://doi.org/10.1016/j.cattod.2016.04.039
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  • ⦁ Clarke, B.O., Anumol, T., Barlaz, M., Snyder, S.A., 2015. Investigating landfill leachate as a source of trace organic pollutants. Chemosphere 127, 269–275. https://doi.org/10.1016/j.chemosphere.2015.02.030
  • ⦁ Cui, Y.-H., Chen, Q., Feng, J.-Y., Liu, Z.-Q., 2014. Effectiveness of electrochemical degradation of sulfamethazine on a nanocomposite SnO 2 electrode. RSC Adv. 4, 30471–30479.
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  • ⦁ Cui, Y.H., Xue, W.J., Yang, S.Q., Tu, J.L., Guo, X.L., Liu, Z.Q., 2018. Electrochemical/peroxydisulfate/Fe3+ treatment of landfill leachate nanofiltration concentrate after ultrafiltration. Chem. Eng. J. 353, 208–217. https://doi.org/10.1016/j.cej.2018.07.101
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  • ⦁ Dindas, G.B., Caliskan, Y., Celebi, E.E., Tekbas, M., Bektas, N., Yatmaz, H.C., 2018. Sequential Treatment of Food Industry Wastewater by Electro-Fenton and Electrocoagulation Processes. Int. J. Electrochem. Sci 13, 12349–12359.
  • ⦁ Ding, J., Gao, Q., Wang, Y., Zhao, G., Wang, K., Jiang, J., Li, J., Zhao, Q., 2020. Simulation and prediction of electrooxidation removal of ammonia and its application in industrial wastewater effluent. Water Environ. Res.
  • ⦁ El Kateb, M., Trellu, C., Darwich, A., Rivallin, M., Bechelany, M., Nagarajan, S., Lacour, S., Bellakhal, N., Lesage, G., Héran, M., Cretin, M., 2019. Electrochemical advanced oxidation processes using novel electrode materials for mineralization and biodegradability enhancement of nanofiltration concentrate of landfill leachates. Water Res. 162, 446–455. https://doi.org/10.1016/j.watres.2019.07.005
  • ⦁ Fernandes, A., Labiadh, L., Ciríaco, L., Pacheco, M.J., Gadri, A., Ammar, S., Lopes, A., 2017. Electro-Fenton oxidation of reverse osmosis concentrate from sanitary landfill leachate: Evaluation of operational parameters. Chemosphere 184, 1223–1229. https://doi.org/10.1016/j.chemosphere.2017.06.088
  • ⦁ Furman, O.S., Teel, A.L., Watts, R.J., 2010. Mechanism of base activation of persulfate. Environ. Sci. Technol. 44, 6423–6428.
  • ⦁ Ghauch, A., Tuqan, A.M., 2012. Oxidation of bisoprolol in heated persulfate/H2O systems: kinetics and products. Chem. Eng. J. 183, 162–171.
  • ⦁ Görmez, F., Görmez, Ö.,Yabalak, E. Gözmen, B., 2020. Application of the central composite design to mineralization of olive mill wastewater by the electro/FeII/persulfate oxidation method. SN Applied Sciences, 2:178.
  • ⦁ Guan, Y.-H., Ma, J., Liu, D.-K., Ou, Z., Zhang, W., Gong, X.-L., Fu, Q., Crittenden, J.C., 2018. Insight into chloride effect on the UV/peroxymonosulfate process. Chem. Eng. J. 352, 477–489.
  • ⦁ Guo, Y., Zhou, J., Lou, X., Liu, R., Xiao, D., Fang, C., Wang, Z., Liu, J., 2014. Enhanced degradation of Tetrabromobisphenol A in water by a UV/base/persulfate system: Kinetics and intermediates. Chem. Eng. J. 254, 538–544.
  • ⦁ Han, S., Hassan, S.U., Zhu, Y., Zhang, Shuai, Liu, H., Zhang, Sen, Li, J., Wang, Z., Zhao, C., 2019. Significance of Activated Carbon Fiber as Cathode in Electro/Fe3+/Peroxydisulfate Oxidation Process for Removing Carbamazepine in Aqueous Environment. Ind. Eng. Chem. Res. 58, 19709–19718.
  • ⦁ He, R., Wei, X.M., Tian, B.H., Su, Y., Lu, Y.L., 2015. Characterization of a joint recirculation of concentrated leachate and leachate to landfills with a microaerobic bioreactor for leachate treatment. Waste Manag. 46, 380–388. https://doi.org/10.1016/j.wasman.2015.08.006
  • ⦁ Hou, L., Zhang, H., Xue, X., 2012. Ultrasound enhanced heterogeneous activation of peroxydisulfate by magnetite catalyst for the degradation of tetracycline in water, in: Separation and Purification Technology. https://doi.org/10.1016/j.seppur.2011.06.023
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There are 63 citations in total.

Details

Primary Language English
Journal Section Research Articles
Authors

Senem Yazıcı Guvenc This is me 0000-0002-2877-0977

Gamze Varank This is me 0000-0003-3437-4505

Ahmet Demir This is me 0000-0003-4649-3368

Emine Can Guven This is me 0000-0002-3540-3235

Publication Date October 5, 2021
Submission Date June 30, 2020
Published in Issue Year 2020 Volume: 38 Issue: 4

Cite

Vancouver Yazıcı Guvenc S, Varank G, Demir A, Can Guven E. ENERGY CONSUMPTION AND EFFICIENCY IMPROVEMENT OF ELECTRO-ACTIVATED PERSULFATE PROCESSES: OPTIMIZATION BY CCD FOR TOC REMOVAL FROM LEACHATE CONCENTRATE. SIGMA. 2021;38(4):1791-810.

IMPORTANT NOTE: JOURNAL SUBMISSION LINK https://eds.yildiz.edu.tr/sigma/