APPLICATION OF SEVERAL ADVANCED OXIDATION PROCESSES FOR THE DESTRUCTION OF ORGANICS IN EFFLUENTS OF PTA PRODUCTION

Year 2016, Volume: 17 Issue: 2, 233 - 249, 14.07.2016

Meral Dükkancı , Gönül Gündüz Ayhan Ezdeşir Hilal Aykaç

https://doi.org/10.18038/btda.91904

Abstract

In this study, the efficiency of several advanced oxidation processes such as ultrasonic oxidation, heterogeneous Fenton-like oxidation, ultrasound or UV assisted heterogeneous Fenton-like oxidation, heterogeneous sonophotoFenton oxidation and oxidation with ultrasound+UV light combination was tested for COD reduction in effluents of purified terephthalic acid (PTA) production. The highest COD removal was achieved as 18% when UV light assisted heterogeneous Fenton-like oxidation was applied to PTA manufacturing wastewater in the presence of 5 wt% iron containing TiO₂ catalyst. This combined advanced oxidation process seems to be a promising one to enhance the COD removal when it is used after biological treatment.

Keywords

Advanced oxidation processes, Purified terephthalic acid, Degradation

References

• Chidambara RBB, Ramkumar N, Sıraf AHJ, Chidambaram C. Biodegradation of acetic, benzoic, isophthalic, toluic and terephthalic acids using a mixed culture: Effluents of PTA production Trans. IChemE.,75B:245-56, 1997.
• Zhang Z, Cheng XX, Wan SP, Sun YQ, Zhu SL, Zhao CJ, Pan WY. Degradability of five aromatic compounds in a pilot wastewater treatment system Int. Biodaterioration and Biodegradation., 58:94-8, Anbia M, Salehis S. Synthesis of polyelectrolyte-modified ordered nanoporous carbon for removal of aromatic organic acids from purified terephthalic acid wastewater Chem. Eng. Res. Design. 90:975- , 2012.
• Martin DS. The adsorption of aromatic acids onto the graphite basal surface Surf. Sci. 536:15-23, Daramola MO, Aransiola EF, Adeogun AG. Comparative study of thermophilic and mesophilic anaerobic treatment of purified terephthalic acid (PTA) wastewater Nat. Sci. 3:371-8, 2011.
• Deshmukh NA, Goel VS, Joshi JB, Mathew T. Kinetics of aerobic biological oxidation of purified terephthalic acid plant waste Process Saf. Environ. 83:224-30, 2005.
• Karthik M, Dafale N, Pathe P, Nandy T. Biodegradability enhancement of purified terephthalic acid wastewater by coagulation-flocculation process as pretreatment J. Hazard. Mater. 154:721-30, Verma S, Prasad B, Mishra IM. Pretreatment of petrochemical wastewater by coagulation and flocculation and the sludge characteristics J. Hazard. Mater. 178:1055-64, 2010.
• Bolova E, Gündüz G, Dükkancı M. Heterogeneous Fenton-like Degradation of Orange II in Water using FeZSM-5 Zeolite Catalyst Int. J. Chem. React. Eng. 10(A18): 1-21, 2012.
• Dükkancı M, Gündüz G. Sonolytic Degradation of Butyric Acid in Aqueous Solutions J. Environ. Manage. 129: 564-8, 2013.
• Sponza DT, Oztekin R. Destruction of some more or less hydrophobic PAHs and their toxicities in a petrochemical industry wastewater with sonication in Turkey Bioresource Technol. 101: 8639-48,
• Thiruvenkatachari R, Kwon TO, Jun JC, Balaji S, Matheswaran M, Moon SI. Application of several advanced oxidation processes for the destruction terephthalic acid (TPA) J. Hazard. Mater.142: 14, 2007.
• Wen YZ, Tong SP, Zheng KF, Wang LL, Lv JZ, Lin J. Removal of terephthalic acid in alkalized wastewater by ferric chloride J. Hazard. Mater. B138: 169-72, 2006.
• Shafaei A, Nikazar M, Arami M, Photocatalytic degradation of terephthalic acid using titania and zinc oxide photocatalysts: Comparative study Desalination. 252: 8-16, 2010.
• Chakraborty AK, Rawal SB, Han SY, Chai SY, Lee WI. Enhancement of visible light photocatalytic efficiency of BiOCl/BiO3 by surface modification with WO3 Appl. Catal. A- Gen. :217-23, 2011.
• Pillai KC, Kwon TO, Moon IS. Degradation of wastewater from terephthalic acid manufacturing process bu ozonation catalyzed with Fe2+, H2O2 and UV light: Direct versus indirect ozonation reactions Appl. Catal. B- Environ. 91: 319-28, 2009.
• Laughrey Z, Bear E, Jones R, Tarr MA. Aqueous sonolytic decomposition of polycyclic aromatic hydrocarbons in the presence of additional dissolved species Ultrason. Sonochem. 8: 353-7, 2001.
• Taylor Jr. E, Cook BB, Tarr MA. Dissolved organic matter inhibition of sonochemical degradation of aqueous polycyclic aromatic hydrocarbons Ultrason. Sonochem. 6: 175-83, 1999.
• Manzai B, Okitsu K, Takenaka N, Bandow H, Maeda Y. Sonochemical degradation of various monocyclic aromatic compounds: Relation between hydrophobicities of organic compounds and the decomposition rates Ultrason. Sonochem. 15: 478-83, 2008.
• Deng Y, Zhang K, Chen H, Wu T, Kryzaniak M, Wellons A, Bolla D, Douglas K, Zuo Y. Iron- catalyzed photochemical transformation of benzoic acid in atmospheric liquids: Product identification and reaction mechanisms Atmospheric Environ. 46: 3665-76, 2006.
• Andreozzi R, Marotta R. Removal of benzoic acid in aqueous solution by Fe(III) homogeneous photocatalysis Water Res. 38: 1225-36, 2004.
• Chan AHC, Chan CK, Barford JP, Porter JF. Solar photocatalytic thin film cascade reactor for treatment of benzoic acid containing wastewater Water Res. 37: 1125-35, 2003.
• Mehratra K, Yablonsky GS, Ray AK. Macrokinetic studies for photocatalytic degradation of benzoic acid in immobilized systems Chemosphere. 60: 1427-36, 2005.
• Mrowetz M, Selli E. Photocatalytic degradation of formic and benzoic acids and hydrogen peroxide evolution in TiO2 and ZnO water suspensions J. Photoch. Photobio. A. 180: 15-22, 2006.
• Velegraki T, Mantzavinos D. Conversion of benzoic acid during TiO2-mediated photocatalytic degradation in water Chem. Eng. J. 140: 15-21, 2008.
• Pariente MI, Martinez F, Melero JA, Botas JA, Velekraki J, Xekoukoulotakis NP, Mantzavinos D. Heterogeneous photo-Fenton oxidation of benzoic acid in water: Effect of operating conditions, reaction by-products and coupling with biological treatment Appl. Catal. B- Environ. 85: 24-32, 2008.
• Wenjun L., Di W., Xin S., Lixiong W., Lei S. Removal of organic matter and ammonia nitrogen in azodicarbonamide wastewater by a combination of power ultrasound radiation and hydrogen peroxide Energy, Resources and Environmental Technology 20:754-9, 2012.
• Ye C.S., Latif PA., Inrahim S., Rosli N., Aziz S. Effect of Ultrasonic Irradiation on COD and TSS in Raw Rubber Mill Effluent EnvironmentAsia 3: 32-5, 2010.
• Nair R.P. Treatment of dye wastewater by sonolysis process IJRMEET 2:1-6, 2014.
• Verma IA., Kumari S. Synergistic effects of sonolysis combined with photocatalysis in degradation of industrial wastewater IJESDM 4:10-2, 2013.
• Vassilakis C., Pantidou A., Psillakis E., Kalogerakis N., Mantzavinos D. Sonolyis of natural phenolic compounds in aqueous solutions: degradation pathways and biodegradability Water Res. :3110-8, 2004.
• Saien J., Shahrezaei F. Organic pollutants removal from petroleum refinery wastewater with nanotitania photocatalyst and UV light emission International Journal of Photoenergy Article ID:703074:1-5, 2012.
• Shahrezaei F., Akhbari A., Rostami A. Photodegradation and removal of phenol and phenolic derivatives from petroleum refinery wastewater using nanoparticles of TiO2 Int. J. Energy Environ. :267-74, 2012.
• Schwidder M, Kumar MS, Klementiev K, Pohl MM, Brückner A, Grünert W. Selective reduction of NO with Fe-ZSM-5 catalysts of low Fe content I. Relations between active site structure and catalytic performance J. Catal. 231: 314-30, 2005.
• Long RQ, Yang RT. Fe-ZSM-5 for selective catalytic reduction of NO with NH3: A comparative study of different preparation techniques Catal. Lett. 74: 201-5, 2001.
• Arana J, Diaz G, Saracho MM, Rodriguez JMD, Melian JAH, Pena JP. Maleic acid photocatalytic degradation using Fe/TiO2 catalysts dependence of the degradation mechanism on the Fe catalysts content Appl. Catal. B- Environ. 36: 113-24, 2002.
• Nicolaides CP. A novel family of solid acid catalysts: substantially amorphous or partially crystalline zeolitic materials Appl. Catal. A- Gen. 185: 211-7, 1999.
• Batista MS, Morales MA, Baggio-Saitovich E, Urquieta-Gonzalez EA. Iron species present in Fe/ZSM-5 catalysts-influence of the preparation method Hyperfine Interact. 134: 161-6, 2001.
• Phu NH, Hoa TTK, Tan NV, Thang HV, Ha PL. Characterization and activity of Fe-ZSM-5 catalysts for the total oxidation of phenol in aqueous solutions Appl. Catal. B-Environ. 34: 267-75, Mohamed MM, Ali IO, Eissa NA. Effect of thermal treatment on surface and bulk properties of Fe/ZSM-5 zeolites prepared by different methods Micropor. Mesopor. Mat. 87: 93-102, 2005.
• Heinrich F, Schmidt C, Löffler E, Menzel M, Grünert W. Fe–ZSM-5 Catalysts for the Selective Reduction of NO by Isobutane—The Problem of the Active Sites J. Catal. 212: 157-72, 2002.
• Park J.-H, Choung J.-H, Nam I.-S, Ham S.-W. N2O decomposition over wet- and solid- exchanged Fe-ZSM-5 catalysts. Appl. Catal. B- Environ.78: 342-54, 2008.
• Jamalluddin NA, Abdullah A.Z. Reactive Dye Degradation by Combined Fe(III)/TiO2 Catalyst and Ultrasonic Irradiation: Effect of Fe (III) Loading and Calcination Temperature Ultrason. Sonochem. 18: 669-78, 2011.
• Zhao BX, Shi BC, Zhang XL, Cao X, Zhang Y.Z. Catalytic Wet Hydrogen Peroxide Oxidation of H-acid in Aqueous Solution with TiO(2)-CeO(2) and Fe/TiO(2)-CeO() Catalysts Desalination. 268: 55- , 2011.
• Jiefang Z, Qiaorong S, Wei Z, Bin H, Jinlong Z, Anpo M., Characterization and Photocatalytic reactivity www.paper.edu.cn/download/downPaper/200312-45. photocatalysts synthesized by hydrothermal method ,
• Khalid NR, Ahmed E, Ikram M, Ahmed M, Phoenix DA, Elhissi A, Ahmed W, Jackson MS. Effects of Calcination on structural Photocatalytic Properties of TiO2 Nanopowders via TiCl4 Hydrolysis J. Mater. Eng. Perform. 22: 371-5, 2013.
• Dükkancı M, Gündüz G, Yılmaz S, Prihod’ko RV. Heterogeneous Fenton-like Degradation of Rhodamine 6G in Water Using CuFeZSM-5 Zeolite Catalyst Prepared by Hydrothermal Synthesis J. Hazard. Mater. 181: 343-50, 2010.
• Dükkancı M, Gündüz G, Yılmaz S, Yaman YC, Prikhod’ko RV, Stolyarova IV. Characterization and Catalytic Activity of CuFeZSM-5 Catalysts for Oxidative Degradation of Rhodamine 6G in Aqueous Solutions Appl. Catal. B- Environ. 95: 270-8, 2010.
• Bolova E, Gündüz G, Dükkancı M, Yılmaz S, Yaman YC. Fe Containing ZSM-5 Zeolite as Catalyst for Wet Peroxide Oxidation of Orange II Int. J. Chem. React Eng. 9: 1-20, 2011.
• Yaman YC, Gündüz G, Dükkancı M. Degradation of CI Reactive Red 141 by Heterogeneous Fenton-like Process over Iron Containing ZSM-5 Zeolites Color. Technol. 129: 69-75, 2013.
• Gogate PR, Pandit AB. Sonophotocatalytic reactors for wastewater Treatment: A critical Review AlChE Journal. 50: 1051-79, 2004.
• Zhong X, Royer S, Zhang H, Huang Q, Xiang L, Valange S, Barrault J. Mesoporous Silica Iron- doped as Stable and Efficient Heterogeneous Catalyst for the Degradation of C.I. Acid Orange 7 using Sono–Photo-Fenton Process Sep. Purif. Technol. 80: 163-71, 2011.
• Konstantinou IK, Albanis TA. TiO2-Assisted Photocatalytic Degradation of Azo Dyes in Aqueous Solution: Kinetic and Mechanistic Investigations - A review Appl. Catal. B-Environ. 49: 1-14, 2004.
• Sun S, Ding J, Bao J, Gao C, Zeming Q, Yang X, He B, Li C. Photocatalytic Degradation of Gaseous Toluene on Fe-TiO2 under Visible Light Irradiation: A Study on the Structure, Activity And Deactivation Mechanism Appl. Surf. Scie. 58: 5031-7, 2012.
• Akpan UG, Hameed BH. Parameters Affecting the Photocatalytic Degradation of Dyes using TiO2-Based Photocatalysts: A Review J. Hazard. Mater. 170: 520-9, 2009.
• Feng JY, Wong R SK, Hu X J, Yue P L. Discoloration and Mineralization of Orange II by Using Fe3+-Doped TiO2 and Bentonite Clay-Based Fe Nanocatalysts Catal. Today 98: 441-6, 2004.
• Liu Y, Sun D Z, Cheng L, Li YP. Preparation and Characterization of Fe2O3-CeO-TiO2/Gamma- AlO3 Catalyst for Degradation Dye Wastewater Journal of Environmental Sciences-China 18: 1189- , 2006.
• Souza MCP, Lenzi GG, Colpini LMS, Jorge LMM, Santos OAA. Photocatalytic Discoloration of Reactive Blue 5G Dye In The Presence of Mixed Oxides and with the Addition of Iron and Silver Brazilian J. Chem. Eng. 28: 393-402, 2011.
• Buddee S, Wongnawa S, Sirimahachai U, Puetpaibool W. Recyclable UV and Visible Light Photocatalytically Active Amorphous TiO(2) doped with M (III) ions (M = Cr and Fe) Materials Chemistry and Physics 126: 167-77, 2011.
• Stasinakis AS. Use of Selected Advanced Oxidation Processes (AOPs) for Wastewater Treatment- A Mini Review Global NEST Journal 10: 376-85, 2008.
• Akın-Ünnü B, Gündüz G. and Dükkancı M. Heterogeneous Fenton-like Oxidation of Crystal Violet using an Iron Loaded ZSM-5 Zeolite Desalination and Water Treatment, 57: 11835-49, 2016.
• Munter R. Advanced Oxıdatıon Processes – Current Status and Prospects Proc. Estonian Acad. Sci. Chem., 50: 59–80, 2001.