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Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies

Year 2024, Volume: 10 Issue: 4, 913 - 921, 31.12.2024
https://doi.org/10.28979/jarnas.1559903

Abstract

The growing reliance on radiation in contemporary applications underscores the imperative to safeguard individuals and the environment from harmful consequences. To mitigate the adverse effects of radiation, polymer composites have begun to garner interest from researchers as potential lead-free shielding materials, largely due to their distinctive attributes, including flexibility, lightness, and environmental benignity. In this study, the gamma radiation shielding capacity of polymethyl methacrylate (PMMA) composites reinforced with varying proportions of Ta₂O₅ (5%, 10%, and 20% wt) was investigated through the utilization of Windows version of photon cross sections on a personal computer (WinXCom) software and the Monte Carlo N-Particle 6 (MCNP6) code. The alignment of the WinXCom and MCNP6 results, despite their different methodologies, provides a robust and reliable understanding of the radiation shielding performance of these composites. The present study investigated the radiation attenuation properties of PMMA/Ta₂O₅ composites about shielding coefficients, including mass attenuation coefficients (MAC), half-value layer (HVL), and effective atomic number (Zeff). The findings indicated that all composites demonstrated enhanced shielding performance compared to pure PMMA. The PMMA/20% Ta₂O₅ composite exhibited MAC values of 1.22-, 1.29-, and 1.28-fold greater than those observed in the silicon-based composites. The MAC increase was observed in the PMMA/20% Ta₂O₅ composite at an energy of 81 keV. The PMMA/20% Ta₂O₅ composite demonstrated the most effective radiation shielding properties. In light of these findings, the PMMA/20% Ta₂O₅ composite can be regarded as a flexible, lightweight, and environmentally friendly shielding material, reassuring these composites' reliability in practical applications.

References

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  • D. Cao, Y. Ge, M. Bourham, D. Moneghan, Gamma radiation shielding properties of poly (methyl methacrylate)/Bi2O3 composites, Nuclear Engineering and Technology 52 (11) (2020) 2613–2619.
  • A. M. Shareef, N. A. Abdulzahara, Manufacture of shielding for attenuation ionization ray by the preparation of nano gadolinium oxide with PMMA, NeuroQuantology 19 (8) (2021) 66–69.
  • D. Adlienė, L. Gilys, E. Griškonis, Development and characterization of new tungsten and tantalum-containing composites for radiation shielding in medicine, Nuclear Instruments and Methods in Physics Research B 467 (2020) 21–26.
  • S. Prabhu, S. G. Bubbly, S. B. Gudennavar, Thermal, mechanical and γ-ray shielding properties of micro and nano-Ta2O5 loaded DGEBA epoxy resin composites, Journal of Applied Polymer Science 138 (2021) 246–266.
  • M. Kamislioglu, Research on the effects of bismuth borate glass system on nuclear radiation shielding parameters, Results in Physics 22 (2021) 103844 10 pages.
  • M. S. Eid, I. I. Bondouk, H. M. Saleh, K. M. Omar, M. I. Sayyed, A. M. El-Khatib, M. Elsafi, Implementation of waste silicate glass into composition of ordinary cement for radiation shielding applications, Nuclear Engineering and Technology 54 (2022) 1456–1463.
  • L. Gerward, N. Guilbert, K. B. Jensen, H. Levring, WinXCom-a program for calculating X-ray attenuation coefficients, Radiation Physics and Chemistry 71 (2004) 653–654.
  • T. A. A. Junior, M. S. Nogueira, V. Vivolo, M. P. A. Potiens, L. L. Campos, Mass attenuation coefficients of X-rays in different barite concrete used in radiation protection as shielding against ionizing radiation, Radiation Physics and Chemistry 140 (2017) 349–354.
  • M. E. Mahmoud, A. M. El-Khatib, M. S. Badawi, A. R. Rashad, R. M. El-Sharkawy, A. A. Thabet, Recycled high-density polyethylene plastics added with lead oxide nanoparticles as sustainable radiation shielding materials, Journal of Cleaner Production 176 (2018) 276–287.
  • M. Büyükyıldız, M. Kurudirek, M. Ekici, O. İçelli, Y. Karabul, Determination of radiation shielding parameters of 304L stainless steel specimens from welding area for photons of various gamma-ray sources, Progress in Nuclear Energy 100 (2017) 245–254.
  • K. Verdipoor, A. Alemi, A. Mesbahi, Photon mass attenuation coefficients of a silicon resin loaded with WO3, PbO, and Bi2O3 micro and nano-particles for radiation shielding, Radiation Physics and Chemistry 147 (2018) 85–90.
  • S. Prabhu, S. G. Bubbly, S. B. Gudennavar, Thermal, mechanical and γ‐ray shielding properties of micro‐and nano‐Ta2O5 loaded DGEBA epoxy resin composites, Journal of Applied Polymer Science 138 (44) (2021) 51289 16 pages.
  • M. S. Al‐Buriahi, C. Eke, S. Alomairy, A. Yildirim, H. I. Alsaeedy, C. Sriwunkum, Radiation attenuation properties of some commercial polymers for advanced shielding applications at low energies, Polymers for Advanced Technologies 32 (2021) 2386–2396.
  • R. El-Mallawany, M. I. Sayyed, M. G. Dong, Y. S. Rammah, Simulation of radiation shielding properties of glasses contain PbO, Radiation Physics and Chemistry 151 (2018) 239–252.
Year 2024, Volume: 10 Issue: 4, 913 - 921, 31.12.2024
https://doi.org/10.28979/jarnas.1559903

Abstract

References

  • M. Çağlar, H. Kayacık, Y. Karabul, M. Kılıç, Z. G. Özdemir, O. İçelli, Na2Si3O7/BaO composites for the gamma-ray shielding in medical applications: Experimental, MCNP5, and WinXCom studies, Progress in Nuclear Energy 117 (2019) 103119 11 pages.
  • T. Özdemir, A. Güngör, I. K. Akbay, H. Uzun, Y. Babucçuoglu, Nano lead oxide and EPDM composite for development of polymer-based radiation shielding material: Gamma irradiation and attenuation tests, Radiation Physics and Chemistry 144 (2018) 248–255.
  • M. A. Hosseini, S. Malekie, F. Kazemi, Experimental evaluation of gamma radiation shielding characteristics of polyvinyl alcohol/tungsten oxide composite: A comparison study of micro and nano sizes of the fillers, Nuclear Instruments and Methods in Physics Research Section A 1026 (2022) 166214 6 pages.
  • M. E. Mahmoud, A. M. El-Khatib, M. S. Badawi, A. R. Rashad, R. M. El-Sharkawy, A. A. Thabet, Fabrication, characterization and gamma rays shielding properties of nano and micro lead oxide-dispersed-high density polyethylene composites, Radiation Physics and Chemistry 145 (2018) 160–173.
  • H. Wang, H. Zhang, Y. Su, T. Liu, H. Yu, Y. Yang, X. Li, B. Guo, Preparation and radiation shielding properties of Gd2O3/PEEK composites, Polymer Composites 36 (2015) 651–659.
  • S. Chen, S. Nambiar, Z. Li, E. Osei, J. Darko, W. Zheng, Z. Sun, P. Liu, J. T. W. Yeow, Bismuth oxide-based nanocomposite for high-energy electron radiation shielding, Journal of Material Science 54 (2019) 3023– 3034.
  • T. Bel, C. Arslan, N. Baydogan, Radiation shielding properties of poly (methyl methacrylate)/colemanite composite for the use in mixed irradiation fields of neutrons and gamma rays, Materials Chemistry and Physics 221 (2019) 58–67.
  • D. Cao, Y. Ge, M. Bourham, D. Moneghan, Gamma radiation shielding properties of poly (methyl methacrylate)/Bi2O3 composites, Nuclear Engineering and Technology 52 (11) (2020) 2613–2619.
  • A. M. Shareef, N. A. Abdulzahara, Manufacture of shielding for attenuation ionization ray by the preparation of nano gadolinium oxide with PMMA, NeuroQuantology 19 (8) (2021) 66–69.
  • D. Adlienė, L. Gilys, E. Griškonis, Development and characterization of new tungsten and tantalum-containing composites for radiation shielding in medicine, Nuclear Instruments and Methods in Physics Research B 467 (2020) 21–26.
  • S. Prabhu, S. G. Bubbly, S. B. Gudennavar, Thermal, mechanical and γ-ray shielding properties of micro and nano-Ta2O5 loaded DGEBA epoxy resin composites, Journal of Applied Polymer Science 138 (2021) 246–266.
  • M. Kamislioglu, Research on the effects of bismuth borate glass system on nuclear radiation shielding parameters, Results in Physics 22 (2021) 103844 10 pages.
  • M. S. Eid, I. I. Bondouk, H. M. Saleh, K. M. Omar, M. I. Sayyed, A. M. El-Khatib, M. Elsafi, Implementation of waste silicate glass into composition of ordinary cement for radiation shielding applications, Nuclear Engineering and Technology 54 (2022) 1456–1463.
  • L. Gerward, N. Guilbert, K. B. Jensen, H. Levring, WinXCom-a program for calculating X-ray attenuation coefficients, Radiation Physics and Chemistry 71 (2004) 653–654.
  • T. A. A. Junior, M. S. Nogueira, V. Vivolo, M. P. A. Potiens, L. L. Campos, Mass attenuation coefficients of X-rays in different barite concrete used in radiation protection as shielding against ionizing radiation, Radiation Physics and Chemistry 140 (2017) 349–354.
  • M. E. Mahmoud, A. M. El-Khatib, M. S. Badawi, A. R. Rashad, R. M. El-Sharkawy, A. A. Thabet, Recycled high-density polyethylene plastics added with lead oxide nanoparticles as sustainable radiation shielding materials, Journal of Cleaner Production 176 (2018) 276–287.
  • M. Büyükyıldız, M. Kurudirek, M. Ekici, O. İçelli, Y. Karabul, Determination of radiation shielding parameters of 304L stainless steel specimens from welding area for photons of various gamma-ray sources, Progress in Nuclear Energy 100 (2017) 245–254.
  • K. Verdipoor, A. Alemi, A. Mesbahi, Photon mass attenuation coefficients of a silicon resin loaded with WO3, PbO, and Bi2O3 micro and nano-particles for radiation shielding, Radiation Physics and Chemistry 147 (2018) 85–90.
  • S. Prabhu, S. G. Bubbly, S. B. Gudennavar, Thermal, mechanical and γ‐ray shielding properties of micro‐and nano‐Ta2O5 loaded DGEBA epoxy resin composites, Journal of Applied Polymer Science 138 (44) (2021) 51289 16 pages.
  • M. S. Al‐Buriahi, C. Eke, S. Alomairy, A. Yildirim, H. I. Alsaeedy, C. Sriwunkum, Radiation attenuation properties of some commercial polymers for advanced shielding applications at low energies, Polymers for Advanced Technologies 32 (2021) 2386–2396.
  • R. El-Mallawany, M. I. Sayyed, M. G. Dong, Y. S. Rammah, Simulation of radiation shielding properties of glasses contain PbO, Radiation Physics and Chemistry 151 (2018) 239–252.
There are 21 citations in total.

Details

Primary Language English
Subjects Medical Physics, Radiation Technology
Journal Section Research Article
Authors

Mustafa Çağlar 0000-0002-0106-7683

Publication Date December 31, 2024
Submission Date October 2, 2024
Acceptance Date December 10, 2024
Published in Issue Year 2024 Volume: 10 Issue: 4

Cite

APA Çağlar, M. (2024). Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies. Journal of Advanced Research in Natural and Applied Sciences, 10(4), 913-921. https://doi.org/10.28979/jarnas.1559903
AMA Çağlar M. Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies. JARNAS. December 2024;10(4):913-921. doi:10.28979/jarnas.1559903
Chicago Çağlar, Mustafa. “Performance of PMMA/Ta2O5 Composites As Medical Radiation Shielding: WinXCom and MCNP6 Studies”. Journal of Advanced Research in Natural and Applied Sciences 10, no. 4 (December 2024): 913-21. https://doi.org/10.28979/jarnas.1559903.
EndNote Çağlar M (December 1, 2024) Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies. Journal of Advanced Research in Natural and Applied Sciences 10 4 913–921.
IEEE M. Çağlar, “Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies”, JARNAS, vol. 10, no. 4, pp. 913–921, 2024, doi: 10.28979/jarnas.1559903.
ISNAD Çağlar, Mustafa. “Performance of PMMA/Ta2O5 Composites As Medical Radiation Shielding: WinXCom and MCNP6 Studies”. Journal of Advanced Research in Natural and Applied Sciences 10/4 (December 2024), 913-921. https://doi.org/10.28979/jarnas.1559903.
JAMA Çağlar M. Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies. JARNAS. 2024;10:913–921.
MLA Çağlar, Mustafa. “Performance of PMMA/Ta2O5 Composites As Medical Radiation Shielding: WinXCom and MCNP6 Studies”. Journal of Advanced Research in Natural and Applied Sciences, vol. 10, no. 4, 2024, pp. 913-21, doi:10.28979/jarnas.1559903.
Vancouver Çağlar M. Performance of PMMA/Ta2O5 Composites as Medical Radiation Shielding: WinXCom and MCNP6 Studies. JARNAS. 2024;10(4):913-21.


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