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Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi

Year 2019, Volume: 23 Issue: 2, 356 - 366, 25.08.2019
https://doi.org/10.19113/sdufenbed.467165

Abstract

Bu çalışmada, adsorpsiyon yöntemi ile sulu ortamdan As(V) giderimi için
ham ve yüzeyi modifiye edilmiş pomzanın etkinliği incelenmiştir.
Granüler
destek malzemesi olarak Isparta pomzası kullanılmış ve demir oksit ile
kaplanmıştır. K
atı
sorbentlerinin yapı karakterizasyonunun belirlenmesi için FTIR, XRD ve BET
yüzey alanı analizi yapılmış ve yüzey morfolojisinin gözlenmesi için SEM
görüntüleri kullanılmıştır.
HIP ve DOKIPkatı sorbentleri kullanılarak sulu çözeltiden
As(V) giderimini etkileyen çözelti pH’ı, başlangıç As(V) konsantrasyonu, temas
süresi, adsorbent dozu ve sıcaklık parametreleri incelenmiş ve optimum giderim
koşulları tespit edilmiştir.
DOKIPiçin maksimum As(V) giderimi ve adsorpsiyon kapasitesi
sırasıyla % 95,99±1,43 ve 1,92±0,03 mg/g olarak elde edilmiştir. DOKIP ile
As(V) adsorpsiyonu için ΔH, ΔS ve ΔG termodinamik parametreleri hesaplanmış,
adsorpsiyon prosesinin ekzotermik karakterli olduğu belirlenmiştir.
Deneysel
adsorpsiyon verilerinin
Langmuir, Freundlich ve Dubinin-Radushkevich (D-R)
izotermlerine uygunluğu incelenmiş ve adsorpsiyon
verilerinin Langmuir modeline uyduğu belirlenmiştir.
Yüksek
adsorpsiyon kapasitelerine dayanarak, sulu çözeltilerden As (V)'in
önderiştirilmesi ve gideriminde DOKIPsorbenti umut verici
alternatif bir adsorban olarak önerilmiştir.

References

  • [1] Monique, B., Fritz, H.F., 2003. Arsenic – a Review. Part I: Occurrence, Toxicity, Speciation, Mobility. Acta Hydrochimica et Hydrobiologica, 311(2003), 9–189.
  • [2] Mohan, D., Pittman, C.U., 2007. Review Arsenic removal from water/wastewater using adsorbents—A critical review. Journal of Hazardous Materials, 142(2007), 1–53.
  • [3] Smedley, P.L., Kinniburgh, D.G., 2002. A review of the source, behaviour and distribution of arsenic in natural waters. Applied Geochemistry 17(2002), 517–568.
  • [4] Choong, T.S.Y., Chuah, T.G., Robiah, Y., Koay, F.L.G., Azni, I., 2007. Arsenic Toxicity, health hazards and removal techniques from water: an overview. Desalination, 217(2007), 139-166.
  • [5] Bhattacharya, P., Mukherjee, A.B., Bundshuh, J., Zevenhoven, R., Loeppert, R.H., 2007. Arsenic in Soil and Groundwater Environment. Volume 9, Elsevier.
  • [6] Jain, C.K., Singh, R.D., 2012. Technological options for the removal of arsenic with special reference to South East Asia. Journal of Environmental Management, 107(2012), 1-18 .
  • [7] Song, S., Valdivieso, A.L., Campos, D.J.H., Peng, C., Fernandez, M.G.M., Soto, I.R., 2006. Arsenic removal from high-arsenic water by enhanced coagulation with ferric ions and coarse calcite. Water Research, 40(2006), 364-372.
  • [8] Malik, A.H., Khan, Z.M., Mahmood, Q., Nasreen, S., Bhatti, Z.A., 2009. Perspectives of low cost arsenic remediation of drinking water in Pakistan and other countries. Journal of Hazardous Materials, 168(2009), 1-12.
  • [9] Wang, S., Zhao, X., 2009. On the potential of biological treatment for arsenic contaminated soils and groundwater. Journal of Environmental Management, 90(2009), 2367–2376.
  • [10] Sharma, V.K., Sohn, M., 2009. Aquatic arsenic: Toxicity, speciation, transformations, and remediation. Environment International, 35(2009), 743-759.
  • [11] Pokhrel, D., Viraraghavan, T., 2006. Arsenic removal from an aqueous solution by a modified fungal biomass. Water Research, 40(2006), 549-552.
  • [12] Lai, C.H., Lo, S.L., Chiang, H.L., 2000. Adsorption/desorption properties of copper ions on the surface of iron-coated sand using BET and EDAX analyses. Chemosphere 41(2000), 1249-1255.
  • [13] Lai, C.H., Chen, C.Y., 2001. Removal of metal ions and humic acid from water by iron-coated filter media. Chemosphere 44(2001), 1177-1184.
  • [14] Bekaroğlu, Ş.Ş.K. 2010. Yüzeyleri Modifiye Olmuş Çeşitli Adsorbanlarla Doğal Organik Madde Giderimi. Süleyman Demirel Üniversitesi,Fen Bilimleri Enstitüsü, Doktora Tezi, 284s, Isparta.
  • [15] Funing, L., Daren C., 1982. Rapid spectrophotometric determination of arsenic and phosphorus after development of molybdenum blue complex at room temperature. Analytical Abstracts, 42(1982), 130.
  • [16] Far, L.B., Souri, B., Heidari, M., Khoshnavazi, R., 2012. Evaluation Of Iron And Manganese-Coated Pumice Application For The Removal Of As(V) From Aqueous Solutions. Iranian Journal Of Environmental Health Science & Engineering, 9(2012), 1-9.
  • [17] Oztel, M.D., Akbal, F., Altas, L., 2015. Arsenite Removal By Adsorption Onto İron Oxide-Coated Pumice And Sepiolite. Environmental Earth Sciences, 73(8)(2015), 4461-4471.
  • [18] Chang, Y., Li, C. W., Benjamin, M. M., 1997. Iron oxide-coated media for NOM sorption and particulate filtration. Journal of the American Water Works Association, 89 (5)(1997), 100-113.
  • [19] Indah, S., Helard, D., 2017. Evaluation Of İron And Manganese-Coated Pumice From Sungai Pasak, West Sumatera, Indonesia For The Removal Of Fe (II) And Mn (II) From Aqueous Solutions. Procedia Environmental Sciences, 37(2017), 556-563.
  • [20] Boddu, V. M., Abburi, K., Talbott, J.L., Smith, E.D., Haasch, R. 2008. Removal of arsenic (III) and arsenic (V) from aqueous medium using chitosan-coated biosorbent. Water Research, 42 (3)(2008), 633–642.
  • [21] Ranjan, D., Talat M. ve Hasan, S.H., 2009. Biosorption of Arsenic from Aqueous Solution Using Agricultural Residue ‘Rice Polish’. Journal of Hazardous Materials, 166(2009), 1050–1059.
  • [22] Natale, F.D., Erto, A., Lancia, A., Musmarra, D., 2008. Experimental and Modelling Analysis of As(V) Ions Adsorption on Granular Activated Carbon. Water Research, 42(2008), 2007–2016.
  • [23] Chen, W., Parette, R., Zou,J., Cannon, F.S. ve Dempsey, B.A., 2007. Arsenic Removal by Iron-Modified Activated Carbon. Water Research, 41(2007), 1851–1858.
  • [24] Wang, X., Liu, Y., Zheng, J., 2016. Removal of As(III) and As(V) from water by chitosan and chitosan derivatives: a review. Environmental Science Pollution Research, 23(2016), 13789–13801.
  • [25] Sarı, A., Mendil, D., Tuzen, M., Soylak, M. 2008. Biosorption of Cd(II) and Cr(III) From Aqueous Solution by Moss (Hylocomium splendens) Biomass: Equilibrium, Kinetic and Thermodynamic Studies. Chemical Engineering Journal, 144(2008), 1–9.
  • [26] Karaoglu, H.M., Zor, Ş., Ugurlu, M., 2010. Biosorption of Cr(III) from solutions using vineyard pruning waste. Chemical Engineering Journal, 159(2010), 98–106.
  • [27] Gupta, V.K., Rastogi, A., Nayak, A. 2010. Adsorption Studies on the Removal of Hexavalent Chromium From aqueous Solution Using a Low Cost Fertilizer Ġndustry Waste Material. The Journal of Colloid and Interface Science, 342(2010), 135–141.
  • [28] Langmuir, I., 1918. The adsorption of gases on plane surfaces of glass, mica and platinium. Journal of American Chemical Society, 40, 1361–1403.
  • [29] Freundlich, H.M.F., 1906. Über die adsorption in lösungen. Zeitschrift für Physikalische Chemie (Leipzig) 57A, 385–470.
  • [30] Dubinin, M.M., Zaverina, E.D., Radushkevich, L.V., 1947. Sorption and structure of active carbons. I. Adsorption of organic vapors, Zhurnal Fizicheskoi Khimii. 21, 1351–1362.
  • [31] Helfferich, F., 1962. Ion Exchange, McGraw Hill, New York, USA, p. 166.
  • [32] Sawalha, M.F., Videa, J.R.P., Gonzalez, J.R., Gardea-Torresdey, J.L., 2006. Biosorption of Cd(II), Cr(III), and Cr(VI) by saltbush (Atriplex canescens) biomass: thermodynamic and isotherm studies. Journal of Colloid and Interface Science, 300, 100–104.
  • [33] Yazdani, M., Tuudjarvi, T., Bhatnagar, A., Vahala, R., 2016. Adsorptive removal of arsenic (V) from aqueous phase by feldspars: Kinetics, mechanism, and thermodynamic aspects of adsorption. Journal of Molecular Liquids, 214(2016), 149–156.
  • [34] Afzali, D., Rouhani, M., Fathirad, F., Shamspur, T., Mostafavi, A., 2016. Nano-iron Oxide Coated On Sand As A New Sorbent For Removal Of Arsenic From Drinking Water. Desalination and Water Treatment, 57(2016), 13030–13037.
  • [35] Chaudhry, S.A., Ahmed, M., Siddiqui, S.I., Ahmed, S., 2016. Fe (III)-Sn (IV) Mixed Binary Oxide-coated Sand Preparation and Its Use for the Removal of As (III) and As (V) from Water: Application of Isotherm, Kinetic and Thermodynamics. Journal of Molecular Liquids, 224(2016), 431–441.
  • [36] Hsu, J.C., Lin, C.J., Liao, C.H., Chen, S.T., 2008. Removal of As (V) and As (III) by Reclaimed Iron-oxide Coated Sands. Journal of Hazardous Materials, 153(2016), 817–826.
  • [37] Massoudinejad, M., Asadi, A., Vosoughi, M., Gholami, M., Karami, M.A.A, 2015. Comprehensive Study (Kinetic, Thermodynamic And Equilibrium) Of Arsenic (V) Adsorption Using KMnO4 Modified Clinoptilolite. Korean Journal of Chemical Engineering, 32(2015), 2078–2086.
  • [38] Yusof, A.M., Malek, N., 2009. Removal of Cr (VI) and As (V) From Aqueous Solutions By HDTMA-Modified Zeolite Y. Journal of Hazardous Materials, 162(2009), 1019–1024.
  • [39] Asere, T.G., Verbeken, K., Tessema, D.A., Fufa, F., Stevens, C.V., Du Laing, G. 2017. Adsorption of As(III) versus As(V) from aqueous solutions by cerium-loaded volcanic rocks. Environmental Science and Pollution Research, 24(25)(2017), 20446-20458.
  • [40] Ouédraogo, I.W.K., Pehlivan, E., Tran, H.T., Paré, S., BonziCoulibaly, Y.L., Zachmann, D., Bahadir, M., 2016. Removal Of Arsenic (V) From Aqueous Medium Using Manganese Oxide Coated Lignocellulose/Silica Adsorbents. Toxicological and Environmental Chemistry, 98(2016), 736–747.
  • [41] Pokhrel, D., Viraraghavan, T., 2008. Arsenic Removal from an Aqueous Solution by Modified A. Niger Biomass: Batch Kinetic and Isotherm Studies. Journal of Hazardous Materials, 150(2008), 818–825.

Removal of Arsenate (V) by Adsorptıon Process from Aqueous Media Using Modified Pumice

Year 2019, Volume: 23 Issue: 2, 356 - 366, 25.08.2019
https://doi.org/10.19113/sdufenbed.467165

Abstract

In this study, the efficiency of row and surface
modified pumice was investigated for As (V) removal from aqueous media by
adsorption method. Isparta pumice is used as granular support material and
coated with iron oxides. FTIR, XRD and BET
surface area analysis were performed for determination of solid sorbents
structure characterization and SEM images were used for observation of surface
morphology.
The
impacts of pH, initial As(V) concentration, contact time, adsorbent dose and
temperature  on As(V) removal were
studied with using HIP and DOKIP as adsorbent and optimum removal conditions
have been determined.  The maximum As(V)
removal and adsorption capacity of DOKIP-1 were 95.99±1.43 % and 1.92±0.03
mg/g, respectively.
The
ΔH, ΔG and ΔS thermodynamic parameters for As(V) adsorption of  DOKIP are calculated and results showed that
the adsorption process has exothermic character.
The Langmuir, Freundlich and Dubinin–Radushkevich (D-R)
isotherms were used to fit the equilibrium data. Langmuir model
resulted in the best fit of the adsorption data.
Based on high adsorption capacities, DOKIP sorbent has
been proposed as a promising alternative adsorbent in the preconcentration and
removal of As (V) from aqueous solutions.

References

  • [1] Monique, B., Fritz, H.F., 2003. Arsenic – a Review. Part I: Occurrence, Toxicity, Speciation, Mobility. Acta Hydrochimica et Hydrobiologica, 311(2003), 9–189.
  • [2] Mohan, D., Pittman, C.U., 2007. Review Arsenic removal from water/wastewater using adsorbents—A critical review. Journal of Hazardous Materials, 142(2007), 1–53.
  • [3] Smedley, P.L., Kinniburgh, D.G., 2002. A review of the source, behaviour and distribution of arsenic in natural waters. Applied Geochemistry 17(2002), 517–568.
  • [4] Choong, T.S.Y., Chuah, T.G., Robiah, Y., Koay, F.L.G., Azni, I., 2007. Arsenic Toxicity, health hazards and removal techniques from water: an overview. Desalination, 217(2007), 139-166.
  • [5] Bhattacharya, P., Mukherjee, A.B., Bundshuh, J., Zevenhoven, R., Loeppert, R.H., 2007. Arsenic in Soil and Groundwater Environment. Volume 9, Elsevier.
  • [6] Jain, C.K., Singh, R.D., 2012. Technological options for the removal of arsenic with special reference to South East Asia. Journal of Environmental Management, 107(2012), 1-18 .
  • [7] Song, S., Valdivieso, A.L., Campos, D.J.H., Peng, C., Fernandez, M.G.M., Soto, I.R., 2006. Arsenic removal from high-arsenic water by enhanced coagulation with ferric ions and coarse calcite. Water Research, 40(2006), 364-372.
  • [8] Malik, A.H., Khan, Z.M., Mahmood, Q., Nasreen, S., Bhatti, Z.A., 2009. Perspectives of low cost arsenic remediation of drinking water in Pakistan and other countries. Journal of Hazardous Materials, 168(2009), 1-12.
  • [9] Wang, S., Zhao, X., 2009. On the potential of biological treatment for arsenic contaminated soils and groundwater. Journal of Environmental Management, 90(2009), 2367–2376.
  • [10] Sharma, V.K., Sohn, M., 2009. Aquatic arsenic: Toxicity, speciation, transformations, and remediation. Environment International, 35(2009), 743-759.
  • [11] Pokhrel, D., Viraraghavan, T., 2006. Arsenic removal from an aqueous solution by a modified fungal biomass. Water Research, 40(2006), 549-552.
  • [12] Lai, C.H., Lo, S.L., Chiang, H.L., 2000. Adsorption/desorption properties of copper ions on the surface of iron-coated sand using BET and EDAX analyses. Chemosphere 41(2000), 1249-1255.
  • [13] Lai, C.H., Chen, C.Y., 2001. Removal of metal ions and humic acid from water by iron-coated filter media. Chemosphere 44(2001), 1177-1184.
  • [14] Bekaroğlu, Ş.Ş.K. 2010. Yüzeyleri Modifiye Olmuş Çeşitli Adsorbanlarla Doğal Organik Madde Giderimi. Süleyman Demirel Üniversitesi,Fen Bilimleri Enstitüsü, Doktora Tezi, 284s, Isparta.
  • [15] Funing, L., Daren C., 1982. Rapid spectrophotometric determination of arsenic and phosphorus after development of molybdenum blue complex at room temperature. Analytical Abstracts, 42(1982), 130.
  • [16] Far, L.B., Souri, B., Heidari, M., Khoshnavazi, R., 2012. Evaluation Of Iron And Manganese-Coated Pumice Application For The Removal Of As(V) From Aqueous Solutions. Iranian Journal Of Environmental Health Science & Engineering, 9(2012), 1-9.
  • [17] Oztel, M.D., Akbal, F., Altas, L., 2015. Arsenite Removal By Adsorption Onto İron Oxide-Coated Pumice And Sepiolite. Environmental Earth Sciences, 73(8)(2015), 4461-4471.
  • [18] Chang, Y., Li, C. W., Benjamin, M. M., 1997. Iron oxide-coated media for NOM sorption and particulate filtration. Journal of the American Water Works Association, 89 (5)(1997), 100-113.
  • [19] Indah, S., Helard, D., 2017. Evaluation Of İron And Manganese-Coated Pumice From Sungai Pasak, West Sumatera, Indonesia For The Removal Of Fe (II) And Mn (II) From Aqueous Solutions. Procedia Environmental Sciences, 37(2017), 556-563.
  • [20] Boddu, V. M., Abburi, K., Talbott, J.L., Smith, E.D., Haasch, R. 2008. Removal of arsenic (III) and arsenic (V) from aqueous medium using chitosan-coated biosorbent. Water Research, 42 (3)(2008), 633–642.
  • [21] Ranjan, D., Talat M. ve Hasan, S.H., 2009. Biosorption of Arsenic from Aqueous Solution Using Agricultural Residue ‘Rice Polish’. Journal of Hazardous Materials, 166(2009), 1050–1059.
  • [22] Natale, F.D., Erto, A., Lancia, A., Musmarra, D., 2008. Experimental and Modelling Analysis of As(V) Ions Adsorption on Granular Activated Carbon. Water Research, 42(2008), 2007–2016.
  • [23] Chen, W., Parette, R., Zou,J., Cannon, F.S. ve Dempsey, B.A., 2007. Arsenic Removal by Iron-Modified Activated Carbon. Water Research, 41(2007), 1851–1858.
  • [24] Wang, X., Liu, Y., Zheng, J., 2016. Removal of As(III) and As(V) from water by chitosan and chitosan derivatives: a review. Environmental Science Pollution Research, 23(2016), 13789–13801.
  • [25] Sarı, A., Mendil, D., Tuzen, M., Soylak, M. 2008. Biosorption of Cd(II) and Cr(III) From Aqueous Solution by Moss (Hylocomium splendens) Biomass: Equilibrium, Kinetic and Thermodynamic Studies. Chemical Engineering Journal, 144(2008), 1–9.
  • [26] Karaoglu, H.M., Zor, Ş., Ugurlu, M., 2010. Biosorption of Cr(III) from solutions using vineyard pruning waste. Chemical Engineering Journal, 159(2010), 98–106.
  • [27] Gupta, V.K., Rastogi, A., Nayak, A. 2010. Adsorption Studies on the Removal of Hexavalent Chromium From aqueous Solution Using a Low Cost Fertilizer Ġndustry Waste Material. The Journal of Colloid and Interface Science, 342(2010), 135–141.
  • [28] Langmuir, I., 1918. The adsorption of gases on plane surfaces of glass, mica and platinium. Journal of American Chemical Society, 40, 1361–1403.
  • [29] Freundlich, H.M.F., 1906. Über die adsorption in lösungen. Zeitschrift für Physikalische Chemie (Leipzig) 57A, 385–470.
  • [30] Dubinin, M.M., Zaverina, E.D., Radushkevich, L.V., 1947. Sorption and structure of active carbons. I. Adsorption of organic vapors, Zhurnal Fizicheskoi Khimii. 21, 1351–1362.
  • [31] Helfferich, F., 1962. Ion Exchange, McGraw Hill, New York, USA, p. 166.
  • [32] Sawalha, M.F., Videa, J.R.P., Gonzalez, J.R., Gardea-Torresdey, J.L., 2006. Biosorption of Cd(II), Cr(III), and Cr(VI) by saltbush (Atriplex canescens) biomass: thermodynamic and isotherm studies. Journal of Colloid and Interface Science, 300, 100–104.
  • [33] Yazdani, M., Tuudjarvi, T., Bhatnagar, A., Vahala, R., 2016. Adsorptive removal of arsenic (V) from aqueous phase by feldspars: Kinetics, mechanism, and thermodynamic aspects of adsorption. Journal of Molecular Liquids, 214(2016), 149–156.
  • [34] Afzali, D., Rouhani, M., Fathirad, F., Shamspur, T., Mostafavi, A., 2016. Nano-iron Oxide Coated On Sand As A New Sorbent For Removal Of Arsenic From Drinking Water. Desalination and Water Treatment, 57(2016), 13030–13037.
  • [35] Chaudhry, S.A., Ahmed, M., Siddiqui, S.I., Ahmed, S., 2016. Fe (III)-Sn (IV) Mixed Binary Oxide-coated Sand Preparation and Its Use for the Removal of As (III) and As (V) from Water: Application of Isotherm, Kinetic and Thermodynamics. Journal of Molecular Liquids, 224(2016), 431–441.
  • [36] Hsu, J.C., Lin, C.J., Liao, C.H., Chen, S.T., 2008. Removal of As (V) and As (III) by Reclaimed Iron-oxide Coated Sands. Journal of Hazardous Materials, 153(2016), 817–826.
  • [37] Massoudinejad, M., Asadi, A., Vosoughi, M., Gholami, M., Karami, M.A.A, 2015. Comprehensive Study (Kinetic, Thermodynamic And Equilibrium) Of Arsenic (V) Adsorption Using KMnO4 Modified Clinoptilolite. Korean Journal of Chemical Engineering, 32(2015), 2078–2086.
  • [38] Yusof, A.M., Malek, N., 2009. Removal of Cr (VI) and As (V) From Aqueous Solutions By HDTMA-Modified Zeolite Y. Journal of Hazardous Materials, 162(2009), 1019–1024.
  • [39] Asere, T.G., Verbeken, K., Tessema, D.A., Fufa, F., Stevens, C.V., Du Laing, G. 2017. Adsorption of As(III) versus As(V) from aqueous solutions by cerium-loaded volcanic rocks. Environmental Science and Pollution Research, 24(25)(2017), 20446-20458.
  • [40] Ouédraogo, I.W.K., Pehlivan, E., Tran, H.T., Paré, S., BonziCoulibaly, Y.L., Zachmann, D., Bahadir, M., 2016. Removal Of Arsenic (V) From Aqueous Medium Using Manganese Oxide Coated Lignocellulose/Silica Adsorbents. Toxicological and Environmental Chemistry, 98(2016), 736–747.
  • [41] Pokhrel, D., Viraraghavan, T., 2008. Arsenic Removal from an Aqueous Solution by Modified A. Niger Biomass: Batch Kinetic and Isotherm Studies. Journal of Hazardous Materials, 150(2008), 818–825.
There are 41 citations in total.

Details

Primary Language Turkish
Subjects Engineering
Journal Section Articles
Authors

Bülent Kırkan 0000-0003-3462-0681

Mustafa Bekaroğlu This is me 0000-0003-3696-1391

Publication Date August 25, 2019
Published in Issue Year 2019 Volume: 23 Issue: 2

Cite

APA Kırkan, B., & Bekaroğlu, M. (2019). Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi. Süleyman Demirel Üniversitesi Fen Bilimleri Enstitüsü Dergisi, 23(2), 356-366. https://doi.org/10.19113/sdufenbed.467165
AMA Kırkan B, Bekaroğlu M. Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi. J. Nat. Appl. Sci. August 2019;23(2):356-366. doi:10.19113/sdufenbed.467165
Chicago Kırkan, Bülent, and Mustafa Bekaroğlu. “Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi Ile Arsenat (V) Giderimi”. Süleyman Demirel Üniversitesi Fen Bilimleri Enstitüsü Dergisi 23, no. 2 (August 2019): 356-66. https://doi.org/10.19113/sdufenbed.467165.
EndNote Kırkan B, Bekaroğlu M (August 1, 2019) Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi. Süleyman Demirel Üniversitesi Fen Bilimleri Enstitüsü Dergisi 23 2 356–366.
IEEE B. Kırkan and M. Bekaroğlu, “Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi”, J. Nat. Appl. Sci., vol. 23, no. 2, pp. 356–366, 2019, doi: 10.19113/sdufenbed.467165.
ISNAD Kırkan, Bülent - Bekaroğlu, Mustafa. “Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi Ile Arsenat (V) Giderimi”. Süleyman Demirel Üniversitesi Fen Bilimleri Enstitüsü Dergisi 23/2 (August 2019), 356-366. https://doi.org/10.19113/sdufenbed.467165.
JAMA Kırkan B, Bekaroğlu M. Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi. J. Nat. Appl. Sci. 2019;23:356–366.
MLA Kırkan, Bülent and Mustafa Bekaroğlu. “Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi Ile Arsenat (V) Giderimi”. Süleyman Demirel Üniversitesi Fen Bilimleri Enstitüsü Dergisi, vol. 23, no. 2, 2019, pp. 356-6, doi:10.19113/sdufenbed.467165.
Vancouver Kırkan B, Bekaroğlu M. Modifiye Edilmiş Pomza Kullanılarak Sulu Ortamlardan Adsorpsiyon Prosesi ile Arsenat (V) Giderimi. J. Nat. Appl. Sci. 2019;23(2):356-6.

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