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Toxic-Free Environment: Forever Chemicals Removal from Water and Wastewater

Yıl 2024, Cilt: 4 Sayı: 2, 122 - 142, 03.10.2024
https://doi.org/10.59838/etoxec.1538643

Öz

Per- and polyfluoroalkyl substances (PFAS), commonly known as "forever chemicals," are persistent synthetic compounds that have been widely utilized since the mid-20th century across various industries. Due to their environmental persistence and potential health risks, PFAS has become a significant concern, particularly in relation to water and wastewater contamination. This paper investigates the complex challenges associated with PFAS, focusing on existing regulatory frameworks, treatment strategies, and innovative clean technologies that aim to reduce or eliminate these harmful substances. The study emphasizes the importance of advanced treatment methods such as electrochemical degradation, nanofiltration, adsorption, and biodegradation, each offering varying degrees of success. Despite advancements in treatment technologies, prevention remains the most effective strategy to minimize PFAS pollution. The paper calls for collaborative efforts from regulatory bodies, industries, and communities to implement more sustainable practices, ensuring a toxic-free environment and aligning with circular economy principles. Continuous research and international cooperation are crucial for developing effective long-term solutions to address PFAS contamination and safeguard both public health and the environment.

Kaynakça

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Toksik Madde-Fre Serbest Ortam: Suyun ve Atıksuların Sonsuz Kimyasallardan Arındırılması

Yıl 2024, Cilt: 4 Sayı: 2, 122 - 142, 03.10.2024
https://doi.org/10.59838/etoxec.1538643

Öz

Per- ve polifluoroalkil maddeler (PFAS), yaygın olarak "sonsuz kimyasallar" olarak bilinen, 20. yüzyılın ortalarından itibaren çeşitli endüstrilerde geniş çapta kullanılan kalıcı sentetik bileşiklerdir. Çevresel kalıcılıkları ve potansiyel sağlık riskleri nedeniyle, PFAS özellikle su ve atık su kirliliğiyle ilgili olarak önemli bir endişe kaynağı haline gelmiştir. Bu makale, mevcut düzenleyici çerçeveler, arıtma stratejileri ve bu zararlı maddeleri azaltmayı veya ortadan kaldırmayı hedefleyen yenilikçi temiz teknolojiler üzerine odaklanarak PFAS ile ilgili karmaşık zorlukları incelemektedir. Çalışma, elektrokimyasal bozunma, nanofiltrasyon, adsorpsiyon ve biyolojik bozunma gibi gelişmiş arıtma yöntemlerinin önemini vurgulamaktadır ve her birinin farklı derecelerde başarı sunduğunu ortaya koymaktadır. Arıtma teknolojilerindeki ilerlemelere rağmen, PFAS kirliliğini en aza indirmek için en etkili strateji, önleme olmaya devam etmektedir. Makale, toksik olmayan bir çevrenin sağlanması ve döngüsel ekonomi ilkeleriyle uyumlu daha sürdürülebilir uygulamaların hayata geçirilmesi için düzenleyici organlar, sanayi ve toplulukların ortak çabalarını gerektirdiğini belirtmektedir. PFAS kirliliğini ele almak ve hem halk sağlığını hem de çevreyi korumak için etkili uzun vadeli çözümler geliştirmek adına sürekli araştırma ve uluslararası iş birliği kritik öneme sahiptir.

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  • Q. Zhuo et al., "Degradation of perfluorinated compounds on a boron-doped diamond electrode," Electrochimica Acta, vol. 77, pp. 17-22, 2012.
  • L. Shi et al., "A review of electrooxidation systems treatment of poly-fluoroalkyl substances (PFAS): electrooxidation degradation mechanisms and electrode materials," Environmental Science and Pollution Research, pp. 1-21, 2024.
  • J. Niu, Y. Li, E. Shang, Z. Xu, and J. Liu, "Electrochemical oxidation of perfluorinated compounds in water," Chemosphere, vol. 146, pp. 526-538, 2016.
  • S. Singh, K. J. Shah, N. Mehta, V. C. Srivastava, and S.-L. Lo, "Electrochemical oxidation of perfluorooctanoic acid (PFOA) from aqueous solution using non-active Ti/SnO2-Sb2O5/PbO2 anodes," Advances in Wastewater Treatment II, vol. 102, p. 48, 2021.
  • F. Yu, Y. Zhang, Y. Zhang, Y. Gao, and Y. Pan, "Promotion of the degradation perfluorooctanoic acid by electro-Fenton under the bifunctional electrodes: Focusing active reaction region by Fe/N co-doped graphene modified cathode," Chemical Engineering Journal, vol. 457, p. 141320, 2023.
  • B. Yang et al., "Electrochemical mineralization of perfluorooctane sulfonate by novel F and Sb co-doped Ti/SnO2 electrode containing Sn-Sb interlayer," Chemical Engineering Journal, vol. 316, pp. 296-304, 2017.
  • T. M. Adeniji and K. J. Stine, "Nanostructure modified electrodes for electrochemical detection of contaminants of emerging concern," Coatings, vol. 13, no. 2, p. 381, 2023.
  • J. N. Uwayezu, I. Carabante, P. van Hees, P. Karlsson, and J. Kumpiene, "Combining electrochemistry and ultraviolet radiation for the degradation of per-and poly-fluoroalkyl substances in contaminated groundwater and wastewater," Journal of Water Process Engineering, vol. 54, p. 104028, 2023.
  • A. M. Pillai and T. Arfin, "Environmental Electrocatalysis for Air Pollution Applications," Electrocatalytic Materials for Renewable Energy, pp. 303-331, 2024.
  • D. J. Liwara et al., "Synthesis of n-isomers: Native and deuterium-labelled short-chain perfluoroalkane sulfonamide derivatives," Journal of Fluorine Chemistry, vol. 278, p. 110311, 2024.
  • L. Zhang et al., "Persulfate activation for efficient remediation of perfluorooctanoic acid (PFOA) and perfluorooctane sulfonic acid (PFOS) in water: Mechanisms, removal efficiency, and future prospects," Journal of Environmental Chemical Engineering, p. 111422, 2023.
  • J.-S. Yang, W. W.-P. Lai, S. C. Panchangam, and A. Y.-C. Lin, "Photoelectrochemical degradation of perfluorooctanoic acid (PFOA) with GOP25/FTO anodes: Intermediates and reaction pathways," Journal of hazardous materials, vol. 391, p. 122247, 2020.
  • R. Xu et al., "Effects of perfluorooctanoic acid (PFOA) and perfluorooctane sulfonic acid (PFOS) on soil microbial community," Microbial ecology, pp. 1-13, 2022.
  • S. J. Smith, "Innovative treatment technologies for PFAS-contaminated water," ed: Diss. Swedish University of Agricultural Sciences. https://doi. org/10.54612 …, 2023.
  • G. Torres-Farradá, S. Thijs, F. Rineau, G. Guerra, and J. Vangronsveld, "White rot fungi as tools for the bioremediation of xenobiotics: a review," Journal of Fungi, vol. 10, no. 3, p. 167, 2024.
  • E. W. Tow et al., "Managing and treating per‐and polyfluoroalkyl substances (PFAS) in membrane concentrates," AWWA water science, vol. 3, no. 5, p. e1233, 2021.
  • A. Berhanu, I. Mutanda, J. Taolin, M. A. Qaria, B. Yang, and D. Zhu, "A review of microbial degradation of per-and polyfluoroalkyl substances (PFAS): Biotransformation routes and enzymes," Science of the Total Environment, vol. 859, p. 160010, 2023.
  • E. Shahsavari, D. Rouch, L. S. Khudur, D. Thomas, A. Aburto-Medina, and A. S. Ball, "Challenges and current status of the biological treatment of PFAS-contaminated soils," Frontiers in Bioengineering and Biotechnology, vol. 8, p. 602040, 2021.
  • D. Grgas, A. Petrina, T. Štefanac, D. Bešlo, and T. Landeka Dragičević, "A review: Per-and polyfluoroalkyl substances—Biological degradation," Toxics, vol. 11, no. 5, p. 446, 2023.
  • S. J. Smith, C. Keane, L. Ahrens, and K. Wiberg, "Integrated Treatment of Per-and Polyfluoroalkyl Substances in Existing Wastewater Treatment Plants─ Scoping the Potential of Foam Partitioning," ACS Es&t Engineering, vol. 3, no. 9, pp. 1276-1285, 2023.
  • T. Zhou et al., "Occurrence, fate, and remediation for per-and polyfluoroalkyl substances (PFAS) in sewage sludge: A comprehensive review," Journal of Hazardous Materials, vol. 466, p. 133637, 2024.
  • S. Chetverikov, G. Hkudaygulov, D. Sharipov, S. Starikov, and D. Chetverikova, "Biodegradation Potential of C7-C10 Perfluorocarboxylic Acids and Data from the Genome of a New Strain of Pseudomonas mosselii 5 (3)," Toxics, vol. 11, no. 12, p. 1001, 2023.
Toplam 124 adet kaynakça vardır.

Ayrıntılar

Birincil Dil İngilizce
Konular Çevre Yönetimi (Diğer), Ekotoksikoloji
Bölüm Derlemeler
Yazarlar

Nada A A Jaradat 0009-0001-1473-7439

Yüksel Orhan Ardalı 0000-0003-1648-951X

Yayımlanma Tarihi 3 Ekim 2024
Gönderilme Tarihi 26 Ağustos 2024
Kabul Tarihi 1 Ekim 2024
Yayımlandığı Sayı Yıl 2024 Cilt: 4 Sayı: 2

Kaynak Göster

IEEE N. A. A. Jaradat ve Y. Orhan Ardalı, “Toxic-Free Environment: Forever Chemicals Removal from Water and Wastewater”, Etoxec, c. 4, sy. 2, ss. 122–142, 2024, doi: 10.59838/etoxec.1538643.