In this study, we developed a nanoplasmonic-based sensor design, which was constructed with a bio-inspired silk material and plasmonic materials (gold nanoparticles). We characterized this mutual integration at molecular level by using Atomic Force Microscopy, Scanning Electron Microscopy, as well as the chemical composition was confirmed with Attenuated Total Reflectance-Fourier Transform Infrared Spectroscopy and X-Ray Photoelectron Spectroscopy analyses, along with contact angle measurements for hydrophilicity/hydrophobicity evaluation. Once a single layer of silk-gold nanoparticle mixture was accomplished, we serially applied an adlayer and plasmonic material to create more sensitive surface. Accordingly, we benchmarked the performance of the multi-layer sensor system, and observed ~6.8 times (or red-shifts from 7.93 nm to 12.90 nm) signal improvements compared to the one developed by a single layer. In sum, we here presented (i) a facile drop-casting method for developing a nanoplasmonic sensor design, (ii) the use of inexpensive off-the-shelf plastic as a substrate, (iii) easy-to-adapt strategy with standard spectrometer devices, and (iv) minimum training for its proper use.
TÜBİTAK; TÜBİTAK; TÜBA; BİLİM AKADEMİSİ
118C254; 120Z335; TÜBA-GEBİP; BAGEP
Dr. Fatih Inci gratefully acknowledges the support from TÜBİTAK 2232-International Fellowship for Outstanding Researchers (Project No: 118C254), TÜBİTAK 3501-Career Development Program (CAREER) (Project No: 120Z335), and Turkish Academy of Sciences - Outstanding Young Scientists Award Program (TÜBA-GEBİP). This publication has been produced benefiting from the 2232 International Fellowship for Outstanding Researchers Program of TÜBİTAK (Project No: 118C254). However, the entire responsibility of the publication/paper belongs to the owner of the publication/paper. The financial support received from TÜBİTAK does not mean that the content of the publication is approved in a scientific sense by TÜBİTAK. This work was supported by the BAGEP Award of the Science Academy.
118C254; 120Z335; TÜBA-GEBİP; BAGEP
Primary Language | English |
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Subjects | Engineering |
Journal Section | Articles |
Authors | |
Project Number | 118C254; 120Z335; TÜBA-GEBİP; BAGEP |
Publication Date | February 28, 2022 |
Acceptance Date | January 28, 2022 |
Published in Issue | Year 2022 Volume: 50 Issue: 2 |
HACETTEPE JOURNAL OF BIOLOGY AND CHEMİSTRY
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