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Farklı Derinliklerdeki Toprak Örneklerinin Radon Salınım Hızlarının Belirlenmesine Yönelik Ön Çalışma

Yıl 2023, Cilt: 25 Sayı: 74, 505 - 512, 15.05.2023
https://doi.org/10.21205/deufmd.2023257419

Öz

Kütahya, Türkiye’de bir inşaat alanında toprak yüzeyinden itibaren 20 cm aralıklarla beş farklı derinlikten toplanan toprak örneklerinin radon alan salınım hızı ve kütle salınım hızları E-Perm algıçları kullanılarak belirlenmiştir. Toprak örneklerinin radon konsantrasyonu akümülatör yöntemi kullanılarak belirlenmiştir. Toprak örneklerinin radon konsantrasyonu beş günlük analiz süresinde 34 ± 4,4 Bq.m-3 ile 86 ± 6,8 Bq.m-3 aralığında, ortalama 48,6 ± 5,1 Bq.m-3 olarak ölçülmüştür. Toprak örneklerinin radon alan salınım hızları 233,2 ± 24,4 mBq.m-2.h-1 ortalama ile 163,7 ± 21,3 ve 413,1 ± 32,6 mBq.m-2.h-1 aralığında hesaplanmıştır. Toprak örneklerinin radon kütle salınım hızları 32,9 ± 4,3 ve 83 ± 6,6 mBq.kg-1.h-1 aralığında ortalama 46,9 ± 4,9 mBq.kg-1.h-1 olarak bulunmuştur. Kapalı ortama örnekleme yapılan toprak örneklerinden 6,5 Bq.m-3’lük radon katkısı geldiği tahmin edilmektedir.

Kaynakça

  • [1] UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) 2000. Sources and effects of ionizing radiation Report to the General Assembly, with Scientific Annexes, Volume I: Sources, ANNEX-B. United Nations Publications, New York.
  • [2] Alhamdi, W.A., Abdullah, K.M.S. 2021. Determination of radium and radon exhalation rate as a function of soil depth of Duhok Province – Iraq. Journal of Radiation Research and Applied Sciences, 14, 1687-8507. DOI: 10.1080/16878507.2021.1999719.
  • [3] Wilkening, M. 1990. Radon-Soil to Air, Chapter 5. Studies in Environmental Science, 40, 43-58. DOI: 10.1016/S0166-1116(08)70009-8.
  • [4] Kotrappa, P., Stieff, F. 2009. Radon exhalation rates from building materials using electret ion chamber radon monitors in accumulators. Health Physics, 97, 163-166. DOI: 10.1097/HP.0b013e3181a9ab15.
  • [5] Tabar, E., Yakut, H., Kuş, A. 2018. Measurement of the radon exhalation rate and effective radium concentration in soil samples of southern Sakarya, Turkey. Indoor and Built Environment, 27, 278-288. DOI:10.1177/1420326X16672510.
  • [6] Tawfiq, N., Jaleel, J. 2015. Radon Concentration in Soil and Radon Exhalation Rate at Al-Dora Refinery and Surrounding Area in Baghdad. Detection, 3, 37-44. DOI: 10.4236/detection.2015.34006.
  • [7] Huang, D., Liu, Y., Liu, Y., Song, Y., Hong, C., Li, X. 2022. Identification of sources with abnormal radon exhalation rates based on radon concentrations in underground environments. Science of The Total Environment, 807, 150800. DOI:10.1016/j.scitotenv.2021.150800.
  • [8] Li, P., Sun, Q., Geng, J., Yan, X., Tang, L. 2022. Radon exhalation from temperature treated loess. Science of The Total Environment, 832, 154925. DOI: 10.1016/j.scitotenv.2022.154925.
  • [9] Kumar, M., Kumar, P., Prajith, R., Agrawal, A., Sahoo, B. K. 2022. Radon exhalation potential and natural radioactivity in soil collected from the surrounding area of a thermal power plant. Journal of Radioanal Nuclear Chemistry, 331, 2597–2607. DOI: 10.1007/s10967-022- 08298-x
  • [10] Atyotha, V., Thopan, P., Fungdet, S., Somtua, J. 2022. Radon exhalation rates of soil samples from Khon Kaen Province, Thailand. Mindanao Journal of Science and Technology, 20, 223-235.
  • [11] Aldenkamp, F.J., de Meijer, R.J., Put, L.W., Stoop, P. 1992. An assessment of in situ radon exhalation measurements, and the relation between free and bound exhalation rates. Radiation Protection Dosimetry, 45, 449–45. DOI: 10.1093/rpd/45.1-4.449.
  • [12] Samuelsson, C., Pettersson, H. 1984. Exhalation of 222Rn from porous materials. Radiation Protection Dosimetry, 7, 95–100. DOI: 10.1093/oxfordjournals.rpd.a082971.
  • [13] Samuelsson, C. 1990. The Closed-Can Exhalation Method for Measuring Radon. Journal of Research of the National Institute of Standards and Technology, 95, 167-169. DOI:10.6028/jres.095.019
  • [14] Abo-Elmagd, M. 2014. Radon exhalation rates corrected for leakage and back diffusion – Evaluation of radon chambers and radon sources with application to ceramic tile. Journal of Radiation Research and Applied Sciences, 7, 390-398. DOI: 10.1016/j.jrras.2014.07.001.
  • [15] Chao, C.Y., Tung T.C. 1999. Radon emanation of building material--impact of back diffusion and difference between one-dimensional and three-dimensional tests. Health Phys., 76, 675-681. DOI: 10.1097/00004032-199906000-00011.
  • [16] Kuş, A., Yakut, H., Tabar , E., 2016. Radon exhalation rates and effective radium contents of the soil samples in Adapazarı, Turkey. AIP Conference Proceedings, 1722, 030009. DOI: 10.1063/1.4944132.
  • [17] Baykara, O., Doğru, M., İnceöz, M., Aksoy, E. 2005. Measurements of radon emanation from soil samples in triple-junction of North and East Anatolian active faults systems in Turkey. Radiation Measurements, 39, 209-212. DOI: 10.1016/j.radmeas.2004.04.011.
  • [18] Kurnaz, A., Turhan, Ş., Hançerlioğulları, A., Gören, E., Karataşlı, M., Altıkulaç, A., Erer, A.M., Metin, O. 2020. Natural radioactivity, radon emanating power and mass exhalation rate of environmental soil samples from Karabük province, Turkey. Radiochimica Acta, 108, 573-579. DOI: 10.1515/ract-2019-3188.
  • [19] Kotrappa, P. 2000. Review of E-PERM passive integrating electret ionization chambers for measuring radon in air, thoron in air, radon in water and thoron flux from surfaces and mill tailings. International Radon Symposium (2000), 14, 1-12.
  • [20] Kotrappa, P., Jester, W.A., 1993. Electret ion chamber radon monitors measure dissolved 222Rn in water. Health Phys., 64, 397-405. DOI: 10.1097/00004032-199304000-00007.
  • [21] Kotrappa, P., Dempsey, J. C., Ramsey, R. W., Stieff, L. R. 1990. A practical E-PERM (Electret Passive Environmental Radon Monitor) system for indoor 222Rn measurement, Health Physics, 58, 461-467.
  • [22] UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) 1988. Sources, effects and risks of ionizing radiation. United Nations, New York.
  • [23] Taşer, A. , Uçaryılmaz, S. , Çataroğlu, I., Sofuoğlu, S. C. 2022. Indoor air CO2 concentrations and ventilation rates in two residences in İzmir, Turkey. Environmental Research and Technology , 5 , 172-180.
  • [24] Radyasyon Güvenliği Yönetmeliği, 2000, Resmi Gazete Sayısı: 23999. (https://www.mevzuat.gov.tr/mevzuat?MevzuatNo=5272&MevzuatTur=7&MevzuatTertip=5 ).

A Preliminary Study to Determine the Radon Exhalation Rates of Soil Samples at Different Depths

Yıl 2023, Cilt: 25 Sayı: 74, 505 - 512, 15.05.2023
https://doi.org/10.21205/deufmd.2023257419

Öz

The radon area exhalation rate and mass exhalation rate of the soil samples collected from five different depths from soil surface with 20 cm intervals of a construction site at Kütahya, Turkey was determined by using the E-Perm detectors. Accumulator method is used to determine the radon concentration of the soil samples. Radon concentration of the soil samples were measured between 34 ± 4.4 Bq.m-3 to 86 ± 6.8 Bq.m-3 with an average value of 48.6 ± 5.1 Bq.m-3 for five days analysis time. Radon area exhalation rate of the soil samples were calculated between 163.7 ± 21.3 and 413.1 ± 32.6 mBq.m-2.h-1 with an average of 233.2 ± 24.4 mBq.m-2 .h-1. Radon mass exhalation rate of the soil samples were found between 32.9 ± 4.3 to 83 ± 6.6 mBq.kg-1.h-1 with a mean value of 46.9 ± 4.9 mBq.kg-1.h-1. The radon contribution to the indoor air from soil samples is estimated as 6.5 Bq.m-3.

Kaynakça

  • [1] UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) 2000. Sources and effects of ionizing radiation Report to the General Assembly, with Scientific Annexes, Volume I: Sources, ANNEX-B. United Nations Publications, New York.
  • [2] Alhamdi, W.A., Abdullah, K.M.S. 2021. Determination of radium and radon exhalation rate as a function of soil depth of Duhok Province – Iraq. Journal of Radiation Research and Applied Sciences, 14, 1687-8507. DOI: 10.1080/16878507.2021.1999719.
  • [3] Wilkening, M. 1990. Radon-Soil to Air, Chapter 5. Studies in Environmental Science, 40, 43-58. DOI: 10.1016/S0166-1116(08)70009-8.
  • [4] Kotrappa, P., Stieff, F. 2009. Radon exhalation rates from building materials using electret ion chamber radon monitors in accumulators. Health Physics, 97, 163-166. DOI: 10.1097/HP.0b013e3181a9ab15.
  • [5] Tabar, E., Yakut, H., Kuş, A. 2018. Measurement of the radon exhalation rate and effective radium concentration in soil samples of southern Sakarya, Turkey. Indoor and Built Environment, 27, 278-288. DOI:10.1177/1420326X16672510.
  • [6] Tawfiq, N., Jaleel, J. 2015. Radon Concentration in Soil and Radon Exhalation Rate at Al-Dora Refinery and Surrounding Area in Baghdad. Detection, 3, 37-44. DOI: 10.4236/detection.2015.34006.
  • [7] Huang, D., Liu, Y., Liu, Y., Song, Y., Hong, C., Li, X. 2022. Identification of sources with abnormal radon exhalation rates based on radon concentrations in underground environments. Science of The Total Environment, 807, 150800. DOI:10.1016/j.scitotenv.2021.150800.
  • [8] Li, P., Sun, Q., Geng, J., Yan, X., Tang, L. 2022. Radon exhalation from temperature treated loess. Science of The Total Environment, 832, 154925. DOI: 10.1016/j.scitotenv.2022.154925.
  • [9] Kumar, M., Kumar, P., Prajith, R., Agrawal, A., Sahoo, B. K. 2022. Radon exhalation potential and natural radioactivity in soil collected from the surrounding area of a thermal power plant. Journal of Radioanal Nuclear Chemistry, 331, 2597–2607. DOI: 10.1007/s10967-022- 08298-x
  • [10] Atyotha, V., Thopan, P., Fungdet, S., Somtua, J. 2022. Radon exhalation rates of soil samples from Khon Kaen Province, Thailand. Mindanao Journal of Science and Technology, 20, 223-235.
  • [11] Aldenkamp, F.J., de Meijer, R.J., Put, L.W., Stoop, P. 1992. An assessment of in situ radon exhalation measurements, and the relation between free and bound exhalation rates. Radiation Protection Dosimetry, 45, 449–45. DOI: 10.1093/rpd/45.1-4.449.
  • [12] Samuelsson, C., Pettersson, H. 1984. Exhalation of 222Rn from porous materials. Radiation Protection Dosimetry, 7, 95–100. DOI: 10.1093/oxfordjournals.rpd.a082971.
  • [13] Samuelsson, C. 1990. The Closed-Can Exhalation Method for Measuring Radon. Journal of Research of the National Institute of Standards and Technology, 95, 167-169. DOI:10.6028/jres.095.019
  • [14] Abo-Elmagd, M. 2014. Radon exhalation rates corrected for leakage and back diffusion – Evaluation of radon chambers and radon sources with application to ceramic tile. Journal of Radiation Research and Applied Sciences, 7, 390-398. DOI: 10.1016/j.jrras.2014.07.001.
  • [15] Chao, C.Y., Tung T.C. 1999. Radon emanation of building material--impact of back diffusion and difference between one-dimensional and three-dimensional tests. Health Phys., 76, 675-681. DOI: 10.1097/00004032-199906000-00011.
  • [16] Kuş, A., Yakut, H., Tabar , E., 2016. Radon exhalation rates and effective radium contents of the soil samples in Adapazarı, Turkey. AIP Conference Proceedings, 1722, 030009. DOI: 10.1063/1.4944132.
  • [17] Baykara, O., Doğru, M., İnceöz, M., Aksoy, E. 2005. Measurements of radon emanation from soil samples in triple-junction of North and East Anatolian active faults systems in Turkey. Radiation Measurements, 39, 209-212. DOI: 10.1016/j.radmeas.2004.04.011.
  • [18] Kurnaz, A., Turhan, Ş., Hançerlioğulları, A., Gören, E., Karataşlı, M., Altıkulaç, A., Erer, A.M., Metin, O. 2020. Natural radioactivity, radon emanating power and mass exhalation rate of environmental soil samples from Karabük province, Turkey. Radiochimica Acta, 108, 573-579. DOI: 10.1515/ract-2019-3188.
  • [19] Kotrappa, P. 2000. Review of E-PERM passive integrating electret ionization chambers for measuring radon in air, thoron in air, radon in water and thoron flux from surfaces and mill tailings. International Radon Symposium (2000), 14, 1-12.
  • [20] Kotrappa, P., Jester, W.A., 1993. Electret ion chamber radon monitors measure dissolved 222Rn in water. Health Phys., 64, 397-405. DOI: 10.1097/00004032-199304000-00007.
  • [21] Kotrappa, P., Dempsey, J. C., Ramsey, R. W., Stieff, L. R. 1990. A practical E-PERM (Electret Passive Environmental Radon Monitor) system for indoor 222Rn measurement, Health Physics, 58, 461-467.
  • [22] UNSCEAR (United Nations Scientific Committee on the Effects of Atomic Radiation) 1988. Sources, effects and risks of ionizing radiation. United Nations, New York.
  • [23] Taşer, A. , Uçaryılmaz, S. , Çataroğlu, I., Sofuoğlu, S. C. 2022. Indoor air CO2 concentrations and ventilation rates in two residences in İzmir, Turkey. Environmental Research and Technology , 5 , 172-180.
  • [24] Radyasyon Güvenliği Yönetmeliği, 2000, Resmi Gazete Sayısı: 23999. (https://www.mevzuat.gov.tr/mevzuat?MevzuatNo=5272&MevzuatTur=7&MevzuatTertip=5 ).
Toplam 24 adet kaynakça vardır.

Ayrıntılar

Birincil Dil İngilizce
Bölüm Araştırma Makalesi
Yazarlar

Hakan Cetinkaya 0000-0002-1466-5930

Erken Görünüm Tarihi 12 Mayıs 2023
Yayımlanma Tarihi 15 Mayıs 2023
Yayımlandığı Sayı Yıl 2023 Cilt: 25 Sayı: 74

Kaynak Göster

Vancouver Cetinkaya H. A Preliminary Study to Determine the Radon Exhalation Rates of Soil Samples at Different Depths. DEUFMD. 2023;25(74):505-12.

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