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SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION

Cilt: 31 Sayı: 2 21 Ağustos 2023
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SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION

Öz

The need for energy is rising quickly, and the usage of fossil fuels is contributing to the greenhouse effect and environmental pollution, both of which are raising public concerns. The development of novel electrochemical energy storage techniques as well as the creation of cleaner, more sustainable energies have both become highly researched topics as a result of this condition. New functional materials are being investigated for the advancement of energy storage. High entropy hydroxides (HEH) have lately been emerged as promising electrocatalyst for universal water splitting reactions, which are central for solid oxide fuel cells, hydrogen production and metal-air batteries. In this work, a cost-effective and scalable fabrication method was applied to fabricate several HEH on Nickel foam through single-step electrodeposition technique. Results showed that high-entropy FeCoNiMnOOH exhibits excellent OER activity with a low overpotential of 151 mV at current density of 100 mA cm−2, which is associated with it’s defective structure.

Anahtar Kelimeler

Water Splitting, High Entropy Materials, Energy Storage and Conversion

Kaynakça

  1. Bayraktar, O., Lökçü, E., Ozgur, C., Erdil, T. & Toparli, C. (2022). Effect of synthesis environment on the electrochemical properties of (FeMnCrCoZn)3O4 high-entropy oxides for Li-ion batteries. International Journal of Energy Research 46, 22124–22133. doi: https://doi.org/10.1002/er.8749
  2. Dai, W., Lu, T. & Pan, Y. (2019). Novel and promising electrocatalyst for oxygen evolution reaction based on MnFeCoNi high entropy alloy. Journal of Power Sources 430, 104-111. doi: https://doi.org/10.1016/j.jpowsour.2019.05.030
  3. Erdil, E., Lökçü, E., Yildiz I., Okuyucu, C., Kalay, Y. E., Toparli, C. (2022). Facile Synthesis and Origin of Enhanced Electrochemical Oxygen Evolution Reaction Performance of 2H-Hexagonal Ba2CoMnO6−δ as a New Member in Double Perovskite Oxides. ACS Omega 7(48), 44147–44155. doi: https://doi.org/10.1021/acsomega.2c05627
  4. Liu, P. F., Yin, H., Fu, H.Q., Zu, M.Y., Yang, H.G., Zhao, H. (2020). Activation strategies of water-splitting electrocatalysts. Journal of Materials Chemistry A 8, 10096-10129.doi: https://doi.org/10.1039/D0TA01680B
  5. Lokcu, E. Toparli, C. & Anik, M. (2020). Electrochemical Performance of (MgCoNiZn)1–xLixO High-Entropy Oxides in Lithium-Ion Batteries. ACS Applied Materials Interfaces 12 (21), 23860–23866. doi: https://doi.org/10.1021/acsami.0c03562
  6. Rost, C. M., Sachet, E., Borman, T., Moballegh, A., Dickey, E. C., Hou, ... Maria, J. P. (2015). Entropy-Stabilized Oxides. Nature Communications 6 (1), 8485. doi: https://doi.org/10.1038/ncomms9485
  7. Trotochaud, L., Young, S. L., Ranney, J. K., & Boettcher, S. W. (2014). Nickel–Iron Oxyhydroxide Oxygen-Evolution Electrocatalysts: The Role of Intentional and Incidental Iron Incorporation. Journal of Ameriacan Chemical Society 136 (18), 6744–6753. doi: https://doi.org/10.1021/ja502379c
  8. Wang, T., Chen, H., Yang, Z., Liang, J. & Dai, S. (2020). High-Entropy Perovskite Fluorides: A New Platform for Oxygen Evolution Catalysis. Journal of American Chemical Society 142 (10), 4550–4554. doi: https://doi.org/10.1021/jacs.9b12377
  9. Wang, Q., Li., J., Li., Y., Shao, G., Jia, Z., Shen, B. (2022). Non-Noble Metal-Based Amorphous High-Entropy Oxides as Efficient and Reliable Electrocatalysts for Oxygen Evolution Reaction. Nano Research 15, 8751–8759. doi: https://doi.org/10.1007/s12274-022-4179-8.
  10. Zhou, C., Chen, X., Liu, S., Han, Y., Meng, H., Jiang, Q., ...Zhang, R. (2022). Superdurable Bifunctional Oxygen Electrocatalyst for High-Performance Zinc–Air Batteries. Journal of American Chemical Society 144 (6), 2694–2704. doi: https://doi.org/10.1021/jacs.1c11675

Kaynak Göster

APA
Toparli, C. (2023). SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION. Eskişehir Osmangazi Üniversitesi Mühendislik ve Mimarlık Fakültesi Dergisi, 31(2), 698-704. https://doi.org/10.31796/ogummf.1290574
AMA
1.Toparli C. SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION. ESOGÜ Müh Mim Fak Derg. 2023;31(2):698-704. doi:10.31796/ogummf.1290574
Chicago
Toparli, Cıgdem. 2023. “SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION”. Eskişehir Osmangazi Üniversitesi Mühendislik ve Mimarlık Fakültesi Dergisi 31 (2): 698-704. https://doi.org/10.31796/ogummf.1290574.
EndNote
Toparli C (01 Ağustos 2023) SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION. Eskişehir Osmangazi Üniversitesi Mühendislik ve Mimarlık Fakültesi Dergisi 31 2 698–704.
IEEE
[1]C. Toparli, “SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION”, ESOGÜ Müh Mim Fak Derg, c. 31, sy 2, ss. 698–704, Ağu. 2023, doi: 10.31796/ogummf.1290574.
ISNAD
Toparli, Cıgdem. “SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION”. Eskişehir Osmangazi Üniversitesi Mühendislik ve Mimarlık Fakültesi Dergisi 31/2 (01 Ağustos 2023): 698-704. https://doi.org/10.31796/ogummf.1290574.
JAMA
1.Toparli C. SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION. ESOGÜ Müh Mim Fak Derg. 2023;31:698–704.
MLA
Toparli, Cıgdem. “SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION”. Eskişehir Osmangazi Üniversitesi Mühendislik ve Mimarlık Fakültesi Dergisi, c. 31, sy 2, Ağustos 2023, ss. 698-04, doi:10.31796/ogummf.1290574.
Vancouver
1.Cıgdem Toparli. SYNTHESIS AND CHARACTERIZATION OF HIGH ENTROPY OXY-HYDROXIDES FOR ELECTROCATALYTIC OXYGEN EVOLUTION AND REDUCTION REACTION. ESOGÜ Müh Mim Fak Derg. 01 Ağustos 2023;31(2):698-704. doi:10.31796/ogummf.1290574