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Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications

Year 2025, Volume: 11 Issue: 5, 1312 - 1326, 21.10.2025

Abstract

High performance interface materials (TIMs) were developed using various nanoparticles and paraffin wax. An indigenous test set up was fabricated using aluminium heat sink and copper plates as heating plate for measuring effective thermal contact resistance (Rth, eff) of prepared TIMs to evaluate their thermal performance. Chrome-Alumel thermocouples were used for measuring the temperature. Furthermore a relative study of effective thermal contact resistance of prepared (TIMs) was carried out to evaluate their performance. The nanoparticle chosen for present distinctive study were SiO2, Al2O3, CuO, GO, rGO. The TIM samples were synthesized by blending 6 wt% of assorted nanoparticles in 5 ml base fluid of paraffin wax. They were uniformly mixed using ultra sonicator to create a smooth and fine paste based TIM. The resulting paste (TIMs) was applied as an ultra-thin layer between the copper heater and aluminium sink of the indigenously designed and fabricated test rig. Power inputs for experiments were 25, 50 and 75W. Experimental studies were done at reduced pressure (RP) and full pressure (FP) applied by completely loosening and tightening the screws of the aluminium heat sink. . Addition of (SiO2, Al2O3, CuO, GO and rGO) nanoparticles to the base fluid paraffin wax significantly decreases the effctive thermal resistance to a large extent as the added nano parcticles helps in better heat conduction due to their enhanced total surface area leading to more effcetive heat evacuation. Enhanced results are observed at full pressure, at reduced pressure drastic increment in (Rth, eff) occurs due to improper gap filling. These results significantly depicts the importance of bondline thickness in performance of TIM. Interestingly siliica based TIM gives the best performance of heat transference to ambience at 50 W power input (Rth, eff = 0.460 C/W) and slightly becomes inferior to GO at higher power input. GO based TIM shows the best results at higher power of 75 W, its Rth, eff being 0.510 C/W.

References

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  • 10. Sun Y, He Y, Tang B, Tao C, Ban J, Jiang L. Influence from the types of surface functional groups of RGO on the performances of thermal interface materials. RSC Adv 2017;7:55790. [Crossref]
  • 11. Schacht R, May D, Wunderle B, Wittler O, Gollhardt A, Michel B, et al. Characterization of thermal interface materials to support thermal simulation. 2007. arXiv:0709.1849v1 [Crossref]
  • 12. Tong T, Zhao Y, Delzeit L, Kashani A, Meyyappan M, Majumdar A. Dense vertically aligned multiwalled carbon nanotube arrays as thermal interface materials. IEEE Trans Compon Packag Manuf 2007;30:1. [Crossref]
  • 13. Narumanchi S, Mihalic M, Kelly K, Eesley G. Thermal interface materials for power electronics applications. 11th Intersociety Conference on Thermal and Thermomechanical Phenomena in Electronic Systems IEEE 2008;395-404. [Crossref]
  • 14. Yada S, Oyake T, Sakata M, Shiomi J. Filler-depletion layer adjacent to interface impacts performance of thermal interface material. AIP Adv 2016;6:015117. [Crossref]
  • 15. Guo Y, Yang X, Ruan K, Kong J, Dong M, Zhang J, et al. Reduced Graphene Oxide Heterostructured Silver Nanoparticles Significantly Enhanced Thermal Conductivities in Hot-Pressed Electrospun Polyimide Nanocomposites. ACS Appl Mater Interfaces 2019;11:25465–73. [Crossref]
  • 16. Chung DDL. Thermal Interface Materials. J Mater Eng Perform 2001;10:56-59. [Crossref]
  • 17. Maheshwari SU, Pillai BC, Govindan K, Raja M, Raja A, Pravin MBS, et al. Development of Low Resistance Thermal Interface Material (TIM) Using Nanomaterials. Int J of Eng Sci Inv 2018;2319–6734:39-46.
  • 18. Iqbal SM, Raj CS, Michael JJ, Irfan AM. A Comparative Investigation of Al2O3/H2O, SiO2/H2O and ZrO2/H2O Nanofluid for Heat Transfer Applications. Digest J Nanomater Biostruct 2017;12:255–263.
  • 19. Balan AE, Sharea AA, Lavasani EJ, Tanasa E, Voinea S, Dobrica B et al. Paraffin-Multilayer Graphene Composite for Thermal Management in Electronics.Materials 2023;16:2-11. [Crossref]

Year 2025, Volume: 11 Issue: 5, 1312 - 1326, 21.10.2025

Abstract

References

  • 1. Micheal HB, de sorgo M, John AM. Permalink Machine translation. 2005;US6054198
  • 2. Micheal HB, de sorgo M, John AM. Conformal thermal interface material for electronic components. 2000; US6054198.
  • 3. Prasher R. Thermal interface materials: historical perspective, status, and future directions. Proc IEEE. 2006; 94:1571–1586. [Crossref]
  • 4. Razeeb KM, Dalton E, Cross GLW, Robinson AJ. Present and future thermal interface materials for electronic devices. Int Mater Rev. 2018; 63:1–21. [Crossref]
  • 5. Mao D, Xie J, Sheng G, Ye H, Yuen MM, Fu XZ, Sun R, Wong CP. Aluminum coated spherical particles filled paraffin wax as a phase change thermal interface materials. In: Proceedings of the 18th International Conference on Electronic Packaging Technology ;2017. pp 828–830. [Crossref]
  • 6. Bhanushali S, Ghosh PC, Simon GP, Cheng W. Copper nanowire filled soft elastomer composites for applications as thermal interface materials. Adv Mater Interfaces 2017; 4:1700387. [Crossref]
  • 7. Lv L, Dai W, Yu J, Jiang N, Lin CT. A mini review: application of graphene paper in thermal interface materials. New Carbon Mater. 2021; 36:930–8. [Crossref]
  • 8. Shahil KMF, Balandin AA. Graphene–multilayer graphene nanocomposites as highly efficient thermal interface materials. Nano Lett. 2012; 2:861–7. [Crossref]
  • 9. Park W, Guo Y, Li X, Hu J, Liu L, Ruan X, et al. High-performance thermal interface material based on few-layer graphene composite. J Phys Chem C 2015;119:26753–26759. [Crossref]
  • 10. Sun Y, He Y, Tang B, Tao C, Ban J, Jiang L. Influence from the types of surface functional groups of RGO on the performances of thermal interface materials. RSC Adv 2017;7:55790. [Crossref]
  • 11. Schacht R, May D, Wunderle B, Wittler O, Gollhardt A, Michel B, et al. Characterization of thermal interface materials to support thermal simulation. 2007. arXiv:0709.1849v1 [Crossref]
  • 12. Tong T, Zhao Y, Delzeit L, Kashani A, Meyyappan M, Majumdar A. Dense vertically aligned multiwalled carbon nanotube arrays as thermal interface materials. IEEE Trans Compon Packag Manuf 2007;30:1. [Crossref]
  • 13. Narumanchi S, Mihalic M, Kelly K, Eesley G. Thermal interface materials for power electronics applications. 11th Intersociety Conference on Thermal and Thermomechanical Phenomena in Electronic Systems IEEE 2008;395-404. [Crossref]
  • 14. Yada S, Oyake T, Sakata M, Shiomi J. Filler-depletion layer adjacent to interface impacts performance of thermal interface material. AIP Adv 2016;6:015117. [Crossref]
  • 15. Guo Y, Yang X, Ruan K, Kong J, Dong M, Zhang J, et al. Reduced Graphene Oxide Heterostructured Silver Nanoparticles Significantly Enhanced Thermal Conductivities in Hot-Pressed Electrospun Polyimide Nanocomposites. ACS Appl Mater Interfaces 2019;11:25465–73. [Crossref]
  • 16. Chung DDL. Thermal Interface Materials. J Mater Eng Perform 2001;10:56-59. [Crossref]
  • 17. Maheshwari SU, Pillai BC, Govindan K, Raja M, Raja A, Pravin MBS, et al. Development of Low Resistance Thermal Interface Material (TIM) Using Nanomaterials. Int J of Eng Sci Inv 2018;2319–6734:39-46.
  • 18. Iqbal SM, Raj CS, Michael JJ, Irfan AM. A Comparative Investigation of Al2O3/H2O, SiO2/H2O and ZrO2/H2O Nanofluid for Heat Transfer Applications. Digest J Nanomater Biostruct 2017;12:255–263.
  • 19. Balan AE, Sharea AA, Lavasani EJ, Tanasa E, Voinea S, Dobrica B et al. Paraffin-Multilayer Graphene Composite for Thermal Management in Electronics.Materials 2023;16:2-11. [Crossref]
There are 19 citations in total.

Details

Primary Language English
Subjects Aerodynamics (Excl. Hypersonic Aerodynamics)
Journal Section Articles
Authors

S. Uma Maheshwari This is me

A. Brusly Solomon This is me 0000-0002-0385-0102

G. Thilagavathi This is me

Madhukar Hemamalin This is me 0000-0003-4536-0408

D. Illakkiam This is me 0009-0009-4654-914X

Publication Date October 21, 2025
Submission Date August 10, 2024
Acceptance Date September 13, 2024
Published in Issue Year 2025 Volume: 11 Issue: 5

Cite

APA Maheshwari, S. U., Solomon, A. B., Thilagavathi, G., … Hemamalin, M. (2025). Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications. Journal of Thermal Engineering, 11(5), 1312-1326. https://doi.org/10.14744/thermal.0000997
AMA Maheshwari SU, Solomon AB, Thilagavathi G, Hemamalin M, Illakkiam D. Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications. Journal of Thermal Engineering. October 2025;11(5):1312-1326. doi:10.14744/thermal.0000997
Chicago Maheshwari, S. Uma, A. Brusly Solomon, G. Thilagavathi, Madhukar Hemamalin, and D. Illakkiam. “Highly Viable Nanoparticle Based Thermal Interface Materials (TIM) for Electronics Device Cooling Applications”. Journal of Thermal Engineering 11, no. 5 (October 2025): 1312-26. https://doi.org/10.14744/thermal.0000997.
EndNote Maheshwari SU, Solomon AB, Thilagavathi G, Hemamalin M, Illakkiam D (October 1, 2025) Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications. Journal of Thermal Engineering 11 5 1312–1326.
IEEE S. U. Maheshwari, A. B. Solomon, G. Thilagavathi, M. Hemamalin, and D. Illakkiam, “Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications”, Journal of Thermal Engineering, vol. 11, no. 5, pp. 1312–1326, 2025, doi: 10.14744/thermal.0000997.
ISNAD Maheshwari, S. Uma et al. “Highly Viable Nanoparticle Based Thermal Interface Materials (TIM) for Electronics Device Cooling Applications”. Journal of Thermal Engineering 11/5 (October2025), 1312-1326. https://doi.org/10.14744/thermal.0000997.
JAMA Maheshwari SU, Solomon AB, Thilagavathi G, Hemamalin M, Illakkiam D. Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications. Journal of Thermal Engineering. 2025;11:1312–1326.
MLA Maheshwari, S. Uma et al. “Highly Viable Nanoparticle Based Thermal Interface Materials (TIM) for Electronics Device Cooling Applications”. Journal of Thermal Engineering, vol. 11, no. 5, 2025, pp. 1312-26, doi:10.14744/thermal.0000997.
Vancouver Maheshwari SU, Solomon AB, Thilagavathi G, Hemamalin M, Illakkiam D. Highly viable nanoparticle based Thermal Interface Materials (TIM) for electronics device cooling applications. Journal of Thermal Engineering. 2025;11(5):1312-26.

IMPORTANT NOTE: JOURNAL SUBMISSION LINK http://eds.yildiz.edu.tr/journal-of-thermal-engineering