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1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi

Yıl 2019, Cilt: 34 Sayı: 4, 129 - 138, 31.12.2019
https://doi.org/10.21605/cukurovaummfd.703226

Öz

Bu çalışmada, C1010 çeliğin 1 M HCl çözeltisindeki korozyonuna 1-benzil-3-metilimidazolyum hekzaflorofosfat’ın inhibisyon etkinliği çalışılmıştır. Elektrokimyasal impedans spektroskopi (EIS) ve potansiyodinamik polarizasyon teknikleri kullanılmıştır. Potansiyodinamik polarizasyon sonuçları, anodik ve katodik akım yoğunluklarının inhibitör derişiminin artması ile azaldığını göstermiştir. EIS ölçümlerinden ise artan sıcaklıklarda dahi inhibisyon etkinliklerinin halen yüksek olduğu belirlenmiştir. İnhibitörün metal üzerindeki adsorpsiyon davranışı, Langmiur adsorpsiyon izotermine uymaktadır. Elde edilen tüm sonuçlar, kullanılan inhibitörün C1010 çeliğin asidik ortamdaki korozyonu üzerine %83,5 inhibisyon etkinliğine sahip olduğu göstermektedir.

Kaynakça

  • 1. Ahamad, I., Prasad, R., Quraishi, M.A., 2010. Thermodynamic, Electrochemical and Quantum Chemical Investigation of Some Schiff Bases as Corrosion Inhibitors for Mild Steel in Hydrochloric Acid Solutions, Corrosion Science 52, 933-942.
  • 2. Zhang, G.A., Hou, X.M., Hou, B.S., Liu, H.F., 2019. Benzimidazole Derivatives as Novel Inhibitors for the Corrosion of Mild Steel in Acidic Solution: Experimental and theoretical studies, Journal of Molecular Liquids 278, 413-427.
  • 3. Vengatesh, G., Sundaravadivelu, M., 2019.Non-toxic Bisacodyl as an Effective Corrosion Inhibitor for Mild Steel in 1 M HCl: Thermodynamic, Electrochemical, SEM, EDX, AFM, FT-IR, DFT and Molecular Dynamics Simulation Studies, Journal of Molecular Liquids 287, 110906.
  • 4. Ma, X., Jiang, X., Xia, S., Shan, M., Li, X., Yu, L., Tang, Q., 2016. New Corrosion Inhibitor Acrylamide Methyl Ether for Mild Steel in 1 M HCl, Applied Surface Science 371, 248-257.
  • 5. Ramya, K., Mohan, R., Anupama, K.K., Joseph, A., 2015. Electrochemical and Theoretical Studies on the Synergistic Interaction and Corrosion Inhibition of Alkyl Benzimidazoles and Thiosemicarbazide Pair on Mild Steel in Hydrochloric Acid, Materials Chemistry and Physics 149-150, 632-647.
  • 6. Li, X., Xie, X., Deng, S., Du, G., 2014. Two Phenylpyrimidine Derivatives as New Corrosion Inhibitors for Cold Rolled Steel in Hydrochloric Acid Solution, Corrosion Science 87, 27-39.
  • 7. Guo, Y., Chen, Z., Zuo, Y., Chen, Y., Yang, W., Xu, B., 2018. Ionic Liquids With Two Typical Hydrophobic Anions as Acidic Corrosion Inhibitors, Journal of Molecular Liquids 269, 886-895.
  • 8. Murulana, L.C., Singh, A.K., Shukla, S.K., Kabanda, M.M., Ebenso, E.E., 2012. Experimental and Quantum Chemical Studies of Some Bis(trifluoromethyl-sulfonyl) Imide Imidazolium-Based Ionic Liquids as Corrosion Inhibitors for Mild Steel in Hydrochloric Acid Solution, Ind. Eng. Chem. Res. 51, 13282-13299.
  • 9. Ashassi-Sorkhabi, H., Es’haghi, M., 2009. Corrosion Inhibition of Mild Steel in Acidic Media by [BMIm] Br Ionic liquid, Materials Chemistry and Physics 114, 267-271.
  • 10. Kowsari, E., Payami, M., Amini, R., Ramezanzadeh, B., Javanbakht, M., 2014. Task-specific Ionic Liquid as a New Green Inhibitor of Mild Steel Corrosion, Applied Surface Science 289, 478-486.
  • 11. Singh, D.K., Ebenso, E.E., Singh, M.K., Behera, D., Udayabhanu, G., John, R.P., 2018. Non-toxic Schiff Bases as Efficient Corrosion Inhibitors for Mild Steel in 1 M HCl: Electrochemical, AFM, FE-SEM and Theoretical Studies, Journal of Molecular Liquids 250, 88-99.
  • 12. He, X., Mao, J., Ma, Q., Tang, Y., 2018. Corrosion Inhibition of Perimidine Derivatives for Mild Steel in Acidic Media: Electrochemical and Computational Studies, Journal of Molecular Liquids 269, 260-268.
  • 13. Chen, W., Luo, H.Q., Li, N.B., 2011. Inhibition Effects of 2,5-dimercapto-1,3,4-thiadiazole on the Corrosion of Mild Steel in Sulphuric Acid Solution, Corrosion Science 53, 3356-3365.
  • 14. Hsu, C.H., Mansfeld, F., 2001. Technical Note: Concerning the Conversion of the Constant Phase Element Parameter Yo Into a Capacitance, Corrosion Science 57, 747-748.
  • 15. Fernandes, C.M., Alvarez, L.X., Escarpini dos Santos, N., Barrios, A.C.M., Ponzio, E.A., 2019. Green Synthesis of 1-benzyl-4-phenyl-1H-1,2,3-triazole, its Application as Corrosion Inhibitor for Mild Steel in Acidic Medium and New Approach of Classical Electrochemical Analyses, Corrosion Science 149, 185-194.
  • 16. Bockris, J.O’M., Reddy, A.K.N., Gamboa-Aldeco, M., 2000. Modern Electrochemistry (Second Edition), Kluwer Academic/Plenum Publishers, New York.
  • 17. Qiang, Y., Zhang, S., Tan, B., Chen, S., 2018. Evaluation of Ginkgo Leaf Extract as an Eco-friendly Corrosion Inhibitor of X70 Steel in HCl Solution, Corrosion Science 133, 6-16.
  • 18. Murmu, M., Saha, S.Kr., Murmu, N.C., Banerjee, P., 2019. Effect of Stereochemical Conformation into the Corrosion Inhibitive Behaviour of Double Azomethine Based Schiff Bases on Mild Steel Surface in 1 mol L-1 HCl Medium: An Experimental, Density Functional Theory and Molecular Dynamics Simulation Study, Corrosion Science 146, 134-151.

The Influence of 1-Benzyl-3-Methylimidazolium Hexafluorophosphate on Corrosion of C1010 Steel in Acidic Medium

Yıl 2019, Cilt: 34 Sayı: 4, 129 - 138, 31.12.2019
https://doi.org/10.21605/cukurovaummfd.703226

Öz

In present study, inhibition efficiency of 1-benzyl-3-methylimidazolium hexafluorophosphate was examined in 1 M HCl solution on corrosion of C1010 steel. Electrochemical impedance spectroscopy (EIS) and potentiodynamic polarization methods were realized. Potentiodynamic polarization results revealed that anodic and cathodic current densities were reduced with increase of inhibitor concentration. It was also determined from EIS measurements inhibition efficiencies were still high even increased temperatures. Adsorption behavior of inhibitor on steel obeyed Langmuir adsorption isotherm. The obtained all results demonstrated that used inhibitor had 83.5% inhibition efficiency on corrosion of C1010 steel in acidic medium.

Kaynakça

  • 1. Ahamad, I., Prasad, R., Quraishi, M.A., 2010. Thermodynamic, Electrochemical and Quantum Chemical Investigation of Some Schiff Bases as Corrosion Inhibitors for Mild Steel in Hydrochloric Acid Solutions, Corrosion Science 52, 933-942.
  • 2. Zhang, G.A., Hou, X.M., Hou, B.S., Liu, H.F., 2019. Benzimidazole Derivatives as Novel Inhibitors for the Corrosion of Mild Steel in Acidic Solution: Experimental and theoretical studies, Journal of Molecular Liquids 278, 413-427.
  • 3. Vengatesh, G., Sundaravadivelu, M., 2019.Non-toxic Bisacodyl as an Effective Corrosion Inhibitor for Mild Steel in 1 M HCl: Thermodynamic, Electrochemical, SEM, EDX, AFM, FT-IR, DFT and Molecular Dynamics Simulation Studies, Journal of Molecular Liquids 287, 110906.
  • 4. Ma, X., Jiang, X., Xia, S., Shan, M., Li, X., Yu, L., Tang, Q., 2016. New Corrosion Inhibitor Acrylamide Methyl Ether for Mild Steel in 1 M HCl, Applied Surface Science 371, 248-257.
  • 5. Ramya, K., Mohan, R., Anupama, K.K., Joseph, A., 2015. Electrochemical and Theoretical Studies on the Synergistic Interaction and Corrosion Inhibition of Alkyl Benzimidazoles and Thiosemicarbazide Pair on Mild Steel in Hydrochloric Acid, Materials Chemistry and Physics 149-150, 632-647.
  • 6. Li, X., Xie, X., Deng, S., Du, G., 2014. Two Phenylpyrimidine Derivatives as New Corrosion Inhibitors for Cold Rolled Steel in Hydrochloric Acid Solution, Corrosion Science 87, 27-39.
  • 7. Guo, Y., Chen, Z., Zuo, Y., Chen, Y., Yang, W., Xu, B., 2018. Ionic Liquids With Two Typical Hydrophobic Anions as Acidic Corrosion Inhibitors, Journal of Molecular Liquids 269, 886-895.
  • 8. Murulana, L.C., Singh, A.K., Shukla, S.K., Kabanda, M.M., Ebenso, E.E., 2012. Experimental and Quantum Chemical Studies of Some Bis(trifluoromethyl-sulfonyl) Imide Imidazolium-Based Ionic Liquids as Corrosion Inhibitors for Mild Steel in Hydrochloric Acid Solution, Ind. Eng. Chem. Res. 51, 13282-13299.
  • 9. Ashassi-Sorkhabi, H., Es’haghi, M., 2009. Corrosion Inhibition of Mild Steel in Acidic Media by [BMIm] Br Ionic liquid, Materials Chemistry and Physics 114, 267-271.
  • 10. Kowsari, E., Payami, M., Amini, R., Ramezanzadeh, B., Javanbakht, M., 2014. Task-specific Ionic Liquid as a New Green Inhibitor of Mild Steel Corrosion, Applied Surface Science 289, 478-486.
  • 11. Singh, D.K., Ebenso, E.E., Singh, M.K., Behera, D., Udayabhanu, G., John, R.P., 2018. Non-toxic Schiff Bases as Efficient Corrosion Inhibitors for Mild Steel in 1 M HCl: Electrochemical, AFM, FE-SEM and Theoretical Studies, Journal of Molecular Liquids 250, 88-99.
  • 12. He, X., Mao, J., Ma, Q., Tang, Y., 2018. Corrosion Inhibition of Perimidine Derivatives for Mild Steel in Acidic Media: Electrochemical and Computational Studies, Journal of Molecular Liquids 269, 260-268.
  • 13. Chen, W., Luo, H.Q., Li, N.B., 2011. Inhibition Effects of 2,5-dimercapto-1,3,4-thiadiazole on the Corrosion of Mild Steel in Sulphuric Acid Solution, Corrosion Science 53, 3356-3365.
  • 14. Hsu, C.H., Mansfeld, F., 2001. Technical Note: Concerning the Conversion of the Constant Phase Element Parameter Yo Into a Capacitance, Corrosion Science 57, 747-748.
  • 15. Fernandes, C.M., Alvarez, L.X., Escarpini dos Santos, N., Barrios, A.C.M., Ponzio, E.A., 2019. Green Synthesis of 1-benzyl-4-phenyl-1H-1,2,3-triazole, its Application as Corrosion Inhibitor for Mild Steel in Acidic Medium and New Approach of Classical Electrochemical Analyses, Corrosion Science 149, 185-194.
  • 16. Bockris, J.O’M., Reddy, A.K.N., Gamboa-Aldeco, M., 2000. Modern Electrochemistry (Second Edition), Kluwer Academic/Plenum Publishers, New York.
  • 17. Qiang, Y., Zhang, S., Tan, B., Chen, S., 2018. Evaluation of Ginkgo Leaf Extract as an Eco-friendly Corrosion Inhibitor of X70 Steel in HCl Solution, Corrosion Science 133, 6-16.
  • 18. Murmu, M., Saha, S.Kr., Murmu, N.C., Banerjee, P., 2019. Effect of Stereochemical Conformation into the Corrosion Inhibitive Behaviour of Double Azomethine Based Schiff Bases on Mild Steel Surface in 1 mol L-1 HCl Medium: An Experimental, Density Functional Theory and Molecular Dynamics Simulation Study, Corrosion Science 146, 134-151.
Toplam 18 adet kaynakça vardır.

Ayrıntılar

Birincil Dil Türkçe
Bölüm Makaleler
Yazarlar

Gökmen Sığırcık Bu kişi benim

Yayımlanma Tarihi 31 Aralık 2019
Yayımlandığı Sayı Yıl 2019 Cilt: 34 Sayı: 4

Kaynak Göster

APA Sığırcık, G. (2019). 1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi. Çukurova Üniversitesi Mühendislik-Mimarlık Fakültesi Dergisi, 34(4), 129-138. https://doi.org/10.21605/cukurovaummfd.703226
AMA Sığırcık G. 1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi. cukurovaummfd. Aralık 2019;34(4):129-138. doi:10.21605/cukurovaummfd.703226
Chicago Sığırcık, Gökmen. “1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi”. Çukurova Üniversitesi Mühendislik-Mimarlık Fakültesi Dergisi 34, sy. 4 (Aralık 2019): 129-38. https://doi.org/10.21605/cukurovaummfd.703226.
EndNote Sığırcık G (01 Aralık 2019) 1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi. Çukurova Üniversitesi Mühendislik-Mimarlık Fakültesi Dergisi 34 4 129–138.
IEEE G. Sığırcık, “1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi”, cukurovaummfd, c. 34, sy. 4, ss. 129–138, 2019, doi: 10.21605/cukurovaummfd.703226.
ISNAD Sığırcık, Gökmen. “1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi”. Çukurova Üniversitesi Mühendislik-Mimarlık Fakültesi Dergisi 34/4 (Aralık 2019), 129-138. https://doi.org/10.21605/cukurovaummfd.703226.
JAMA Sığırcık G. 1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi. cukurovaummfd. 2019;34:129–138.
MLA Sığırcık, Gökmen. “1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi”. Çukurova Üniversitesi Mühendislik-Mimarlık Fakültesi Dergisi, c. 34, sy. 4, 2019, ss. 129-38, doi:10.21605/cukurovaummfd.703226.
Vancouver Sığırcık G. 1-Benzil-3-Metilimidazolyum Hekzaflorofosfat’ın Asidik Ortamda C1010 Çeliğin Korozyonuna Etkisi. cukurovaummfd. 2019;34(4):129-38.