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Spin Radikal Katkılama Yoluyla Organik Fotovoltaik Güneş Pillerinin Verimliliğinin Artırılması

Yıl 2024, Cilt: 40 Sayı: 1, 68 - 74, 30.04.2024

Öz

Güneş ışığının absorbesi üzerine, organik fotovoltaiklerde (OPV) eksiton adı verilen uyarılmış bir enerji durumu oluşur. Singlet ve triplet eksitonlar olmak üzere iki tür eksiton vardır. OPV'de güç dönüşüm verimliliği (PCE), singlet eksitonların kısa ömürleri nedeniyle sınırlıdır, çünkü bunlar hızla rekombine olurlar. Bu sorunun üstesinden gelmek için, spin ½ radikali galvinoksili MEH-PPV: PCBM bulk heterojonksiyonuna dahil ederek tripletleri verimli bir şekilde elde ettik. Fotovoltaikler, galvinoxyl içermeyen cihaza kıyasla PCE'de artış göstermektedir. PCE'deki artışın altında yatan mekanizmayı ortaya çıkarmak için, OPV'lerin manyeto-fotokondüktansı (MPC), çeşitli galvinoksil konsantrasyon oranları ile katkılanmış filmler için ölçülmüştür.

Destekleyen Kurum

Erciyes Üniversitesi

Proje Numarası

FBA- 2022-11983

Kaynakça

  • Peet, J., Senatore, M.L., Heeger, A.J. and Bazan, G.C., 2009. The role of processing in the fabrication and optimization of plastic solar cells. Advanced Materials, 21(14‐15), pp.1521-1527.
  • Chen, L.M., Hong, Z., Li, G. and Yang, Y., 2009. Recent progress in polymer solar cells: manipulation of polymer: fullerene morphology and the formation of efficient inverted polymer solar cells. Advanced materials, 21(14‐15), pp.1434-1449.
  • Yang, K., Arif, M., Förster, M., Scherf, U. and Guha, S., 2009. Triplet excitons in a ladder-type conjugated polymer: Application in solar cells. Synthetic metals, 159(21-22), pp.2338-2341.
  • Chang, M.Y., Chen, Y.F., Tsai, Y.S. and Chi, K.M., 2008. Blending platinum nanoparticles into poly (3-hexylthiophene):[6, 6]-phenyl-C61-butyric acid methyl ester enhances the efficiency of polymer solar cells. Journal of the Electrochemical Society, 156(2), p.B234.
  • Tung, V.C., Chen, L.M., Allen, M.J., Wassei, J.K., Nelson, K., Kaner, R.B. and Yang, Y., 2009. Low-temperature solution processing of graphene− carbon nanotube hybrid materials for high-performance transparent conductors. Nano letters, 9(5), pp.1949-1955.
  • Eakins, G.L., Alford, J.S., Tiegs, B.J., Breyfogle, B.E. and Stearman, C.J., 2011. Tuning HOMO–LUMO levels: trends leading to the design of 9‐fluorenone scaffolds with predictable electronic and optoelectronic properties. Journal of Physical Organic Chemistry, 24(11), pp.1119-1128.
  • Du, H., Deng, Z., Lü, Z., Yin, Y., Yu, L., Wu, H., Chen, Z., Zou, Y., Wang, Y., Liu, H. and Li, Y., 2011. The effect of graphdiyne doping on the performance of polymer solar cells. Synthetic metals, 161(19-20), pp.2055-2057.
  • Zhou, M., Wang, B., Jiang, X., Zakhidov, A.A., Ferraris, J.P., Azunskis, D. and Hanley, L., 2011. Synthesis of PbS Nanocrystal/Functionalized Conducting Polymers for Plastic Solar Cells. International Journal of Nanoscience, 10(03), pp.521-532.
  • Zhang, C., Sun, J., Li, R., Sun, S.S., Lafalce, E. and Jiang, X., 2011. Poly (3-dodecylthienylenevinylene) s: Regioregularity and Crystallinity. Macromolecules, 44(16), pp.6389-6396.
  • Gorenflot, J., Sperlich, A., Baumann, A., Rauh, D., Vasilev, A., Li, C., Baumgarten, M., Deibel, C. and Dyakonov, V., 2012. Detailed study of N, N′-(diisopropylphenyl)-terrylene-3, 4: 11, 12-bis (dicarboximide) as electron acceptor for solar cells application. Synthetic metals, 161(23-24), pp.2669-2676.
  • Zeng, W., Yong, K.S., Kam, Z.M., Chen, Z.K. and Li, Y., 2012. Effect of MoO3 as an interlayer on the performance of organic solar cells based on ZnPc and C60. Synthetic metals, 161(23-24), pp.2748-2752.
  • Zhao, Y., Guo, X., Xie, Z., Qu, Y., Geng, Y. and Wang, L., 2009. Solvent vapor‐induced self assembly and its influence on optoelectronic conversion of poly (3‐hexylthiophene): Methanofullerene bulk heterojunction photovoltaic cells. Journal of applied polymer science, 111(4), pp.1799-1804.
  • Yao, Y., Hou, J., Xu, Z., Li, G. and Yang, Y., 2008. Effects of solvent mixtures on the nanoscale phase separation in polymer solar cells. Advanced Functional Materials, 18(12), pp.1783-1789.
  • Perez, M.D., Borek, C., Forrest, S.R. and Thompson, M.E., 2009. Molecular and morphological influences on the open circuit voltages of organic photovoltaic devices. Journal of the American Chemical Society, 131(26), pp.9281-9286.
  • Singh, S., Pandit, B., Basel, T.P., Li, S., Laird, D. and Vardeny, Z.V., 2012. Two-step charge photogeneration dynamics in polymer/fullerene blends for photovoltaic applications. Physical Review B, 85(20), p.205206.
  • Bakulin, A.A., Rao, A., Pavelyev, V.G., van Loosdrecht, P.H., Pshenichnikov, M.S., Niedzialek, D., Cornil, J., Beljonne, D. and Friend, R.H., 2012. The role of driving energy and delocalized states for charge separation in organic semiconductors. Science, 335(6074), pp.1340-1344.
  • Benson‐Smith, J.J., Goris, L., Vandewal, K., Haenen, K., Manca, J.V., Vanderzande, D., Bradley, D.D. and Nelson, J., 2007. Formation of a Ground‐State Charge‐Transfer Complex in Polyfluorene//[6, 6]‐Phenyl‐C61 Butyric Acid Methyl Ester (PCBM) Blend Films and Its Role in the Function of Polymer/PCBM Solar Cells. Advanced Functional Materials, 17(3), pp.451-457.
  • Drori, T., Holt, J. and Vardeny, Z.V., 2010. Optical studies of the charge transfer complex in polythiophene/fullerene blends for organic photovoltaic applications. Physical Review B, 82(7), p.075207.
  • Behrends, J., Sperlich, A., Schnegg, A., Biskup, T., Teutloff, C., Lips, K., Dyakonov, V. and Bittl, R., 2012. Direct detection of photoinduced charge transfer complexes in polymer fullerene blends. Physical Review B, 85(12), p.125206.
  • Ohkita, H., Cook, S., Astuti, Y., Duffy, W., Tierney, S., Zhang, W., Heeney, M., McCulloch, I., Nelson, J., Bradley, D.D. and Durrant, J.R., 2008. Charge carrier formation in polythiophene/fullerene blend films studied by transient absorption spectroscopy. Journal of the American Chemical Society, 130(10), pp.3030-3042.
  • Holt, J., Singh, S., Drori, T., Zhang, Y. and Vardeny, Z.V., 2009. Optical probes of π-conjugated polymer blends with strong acceptor molecules. Physical Review B, 79(19), p.195210.
  • Howard, I.A., Mauer, R., Meister, M. and Laquai, F., 2010. Effect of morphology on ultrafast free carrier generation in polythiophene: fullerene organic solar cells. Journal of the American Chemical Society, 132(42), pp.14866-14876.
  • Coppinger, G.M., 1957. A stable phenoxy radical inert to oxygen. Journal of the American Chemical Society, 79(2), pp.501-502.
  • Kharasch, M.S. and Joshi, B.S., 1957. Reactions of hindered phenols. I. Reactions of 4, 4'-dihydroxy-3, 5, 3', 5'-tetra-tert-butyl diphenylmethane. The Journal of Organic Chemistry, 22(11), pp.1435-1438.
  • Zhang, Y., Basel, T.P., Gautam, B.R., Yang, X., Mascaro, D.J., Liu, F. and Vardeny, Z.V., 2012. Spin-enhanced organic bulk heterojunction photovoltaic solar cells. Nature communications, 3(1), p.1043.
  • Zhang, Y., Gautam, B.R., Basel, T.P., Mascaro, D.J. and Vardeny, Z.V., 2013. Organic bulk heterojunction solar cells enhanced by spin interaction. Synthetic metals, 173, pp.2-9.
  • Wang, Y., Harmon, N.J., Sahin-Tiras, K., Wohlgenannt, M. and Flatté, M.E., 2014. Anomalous organic magnetoresistance from competing carrier-spin-dependent interactions with localized electronic and nuclear spins. Physical Review B, 90(6), p.060204.
  • Yang, S.H., Le Rendu, P., Nguyen, T.P. and Hsu, C.S., 2007. Fabrication of MEH-PPV/SIO2 and MEH-PPV/SIO2 nanocomposites with enhanced luminescent stabilities. Reviews on Advanced Materials Science, 15(2), pp.144-149.
  • Mahmoud, F.A., Elazab, I., Abo-Elenien, O.M., Abdel Fatah, A. and Ahmed, A.A., 2019. Optical characterization of Poly [2-methoxy-5-(2-ethylhexyloxy-p-phenylene vinylene](MEH-PPV): C60, MEH-PPV: C60: TiO2 and MEHPPV: C60: ZnO Thin Films. Egyptian Journal of Chemistry, 62(2), pp.311-323.
  • Zang, H., Xu, Z. and Hu, B., 2010. Magneto-optical investigations on the formation and dissociation of intermolecular charge-transfer complexes at donor− acceptor interfaces in bulk-heterojunction organic solar cells. The Journal of Physical Chemistry B, 114(17), pp.5704-5709.
  • Shakya, P., Desai, P., Kreouzis, T., Gillin, W.P., Tuladhar, S.M., Ballantyne, A.M. and Nelson, J., 2008. The effect of applied magnetic field on photocurrent generation in poly-3-hexylthiophene:[6, 6]-phenyl C61-butyric acid methyl ester photovoltaic devices. Journal of Physics: Condensed Matter, 20(45), p.452203.
  • Lei, Y., Song, Q., Zhang, Y., Chen, P., Liu, R., Zhang, Q. and Xiong, Z., 2009. Magnetoconductance of polymer–fullerene bulk heterojunction solar cells. Organic electronics, 10(7), pp.1288-1292.

Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping

Yıl 2024, Cilt: 40 Sayı: 1, 68 - 74, 30.04.2024

Öz

Upon absorption of the sunlight, an excited energy state called exciton is generated in organic photovoltaics (OPV). There exist two kinds of excitons, singlet and triplet excitons. In OPV, the power conversion efficiency (PCE) is limited by the short lifetime of singlet excitons since they recombine quickly. To overcome this problem, we have introduced the spin ½ radical galvinoxyl into the MEH-PPV: PCBM bulk heterojunction to harvest triplets efficiently. The photovoltaic device shows an enhancement in PCE compared to the device without galvinoxyl. To reveal the underlying mechanism for the increase in PCE, magneto-photoconductance (MPC) of the OPVs was measured for the films, doped with various galvinoxyl concentration rates.

Proje Numarası

FBA- 2022-11983

Kaynakça

  • Peet, J., Senatore, M.L., Heeger, A.J. and Bazan, G.C., 2009. The role of processing in the fabrication and optimization of plastic solar cells. Advanced Materials, 21(14‐15), pp.1521-1527.
  • Chen, L.M., Hong, Z., Li, G. and Yang, Y., 2009. Recent progress in polymer solar cells: manipulation of polymer: fullerene morphology and the formation of efficient inverted polymer solar cells. Advanced materials, 21(14‐15), pp.1434-1449.
  • Yang, K., Arif, M., Förster, M., Scherf, U. and Guha, S., 2009. Triplet excitons in a ladder-type conjugated polymer: Application in solar cells. Synthetic metals, 159(21-22), pp.2338-2341.
  • Chang, M.Y., Chen, Y.F., Tsai, Y.S. and Chi, K.M., 2008. Blending platinum nanoparticles into poly (3-hexylthiophene):[6, 6]-phenyl-C61-butyric acid methyl ester enhances the efficiency of polymer solar cells. Journal of the Electrochemical Society, 156(2), p.B234.
  • Tung, V.C., Chen, L.M., Allen, M.J., Wassei, J.K., Nelson, K., Kaner, R.B. and Yang, Y., 2009. Low-temperature solution processing of graphene− carbon nanotube hybrid materials for high-performance transparent conductors. Nano letters, 9(5), pp.1949-1955.
  • Eakins, G.L., Alford, J.S., Tiegs, B.J., Breyfogle, B.E. and Stearman, C.J., 2011. Tuning HOMO–LUMO levels: trends leading to the design of 9‐fluorenone scaffolds with predictable electronic and optoelectronic properties. Journal of Physical Organic Chemistry, 24(11), pp.1119-1128.
  • Du, H., Deng, Z., Lü, Z., Yin, Y., Yu, L., Wu, H., Chen, Z., Zou, Y., Wang, Y., Liu, H. and Li, Y., 2011. The effect of graphdiyne doping on the performance of polymer solar cells. Synthetic metals, 161(19-20), pp.2055-2057.
  • Zhou, M., Wang, B., Jiang, X., Zakhidov, A.A., Ferraris, J.P., Azunskis, D. and Hanley, L., 2011. Synthesis of PbS Nanocrystal/Functionalized Conducting Polymers for Plastic Solar Cells. International Journal of Nanoscience, 10(03), pp.521-532.
  • Zhang, C., Sun, J., Li, R., Sun, S.S., Lafalce, E. and Jiang, X., 2011. Poly (3-dodecylthienylenevinylene) s: Regioregularity and Crystallinity. Macromolecules, 44(16), pp.6389-6396.
  • Gorenflot, J., Sperlich, A., Baumann, A., Rauh, D., Vasilev, A., Li, C., Baumgarten, M., Deibel, C. and Dyakonov, V., 2012. Detailed study of N, N′-(diisopropylphenyl)-terrylene-3, 4: 11, 12-bis (dicarboximide) as electron acceptor for solar cells application. Synthetic metals, 161(23-24), pp.2669-2676.
  • Zeng, W., Yong, K.S., Kam, Z.M., Chen, Z.K. and Li, Y., 2012. Effect of MoO3 as an interlayer on the performance of organic solar cells based on ZnPc and C60. Synthetic metals, 161(23-24), pp.2748-2752.
  • Zhao, Y., Guo, X., Xie, Z., Qu, Y., Geng, Y. and Wang, L., 2009. Solvent vapor‐induced self assembly and its influence on optoelectronic conversion of poly (3‐hexylthiophene): Methanofullerene bulk heterojunction photovoltaic cells. Journal of applied polymer science, 111(4), pp.1799-1804.
  • Yao, Y., Hou, J., Xu, Z., Li, G. and Yang, Y., 2008. Effects of solvent mixtures on the nanoscale phase separation in polymer solar cells. Advanced Functional Materials, 18(12), pp.1783-1789.
  • Perez, M.D., Borek, C., Forrest, S.R. and Thompson, M.E., 2009. Molecular and morphological influences on the open circuit voltages of organic photovoltaic devices. Journal of the American Chemical Society, 131(26), pp.9281-9286.
  • Singh, S., Pandit, B., Basel, T.P., Li, S., Laird, D. and Vardeny, Z.V., 2012. Two-step charge photogeneration dynamics in polymer/fullerene blends for photovoltaic applications. Physical Review B, 85(20), p.205206.
  • Bakulin, A.A., Rao, A., Pavelyev, V.G., van Loosdrecht, P.H., Pshenichnikov, M.S., Niedzialek, D., Cornil, J., Beljonne, D. and Friend, R.H., 2012. The role of driving energy and delocalized states for charge separation in organic semiconductors. Science, 335(6074), pp.1340-1344.
  • Benson‐Smith, J.J., Goris, L., Vandewal, K., Haenen, K., Manca, J.V., Vanderzande, D., Bradley, D.D. and Nelson, J., 2007. Formation of a Ground‐State Charge‐Transfer Complex in Polyfluorene//[6, 6]‐Phenyl‐C61 Butyric Acid Methyl Ester (PCBM) Blend Films and Its Role in the Function of Polymer/PCBM Solar Cells. Advanced Functional Materials, 17(3), pp.451-457.
  • Drori, T., Holt, J. and Vardeny, Z.V., 2010. Optical studies of the charge transfer complex in polythiophene/fullerene blends for organic photovoltaic applications. Physical Review B, 82(7), p.075207.
  • Behrends, J., Sperlich, A., Schnegg, A., Biskup, T., Teutloff, C., Lips, K., Dyakonov, V. and Bittl, R., 2012. Direct detection of photoinduced charge transfer complexes in polymer fullerene blends. Physical Review B, 85(12), p.125206.
  • Ohkita, H., Cook, S., Astuti, Y., Duffy, W., Tierney, S., Zhang, W., Heeney, M., McCulloch, I., Nelson, J., Bradley, D.D. and Durrant, J.R., 2008. Charge carrier formation in polythiophene/fullerene blend films studied by transient absorption spectroscopy. Journal of the American Chemical Society, 130(10), pp.3030-3042.
  • Holt, J., Singh, S., Drori, T., Zhang, Y. and Vardeny, Z.V., 2009. Optical probes of π-conjugated polymer blends with strong acceptor molecules. Physical Review B, 79(19), p.195210.
  • Howard, I.A., Mauer, R., Meister, M. and Laquai, F., 2010. Effect of morphology on ultrafast free carrier generation in polythiophene: fullerene organic solar cells. Journal of the American Chemical Society, 132(42), pp.14866-14876.
  • Coppinger, G.M., 1957. A stable phenoxy radical inert to oxygen. Journal of the American Chemical Society, 79(2), pp.501-502.
  • Kharasch, M.S. and Joshi, B.S., 1957. Reactions of hindered phenols. I. Reactions of 4, 4'-dihydroxy-3, 5, 3', 5'-tetra-tert-butyl diphenylmethane. The Journal of Organic Chemistry, 22(11), pp.1435-1438.
  • Zhang, Y., Basel, T.P., Gautam, B.R., Yang, X., Mascaro, D.J., Liu, F. and Vardeny, Z.V., 2012. Spin-enhanced organic bulk heterojunction photovoltaic solar cells. Nature communications, 3(1), p.1043.
  • Zhang, Y., Gautam, B.R., Basel, T.P., Mascaro, D.J. and Vardeny, Z.V., 2013. Organic bulk heterojunction solar cells enhanced by spin interaction. Synthetic metals, 173, pp.2-9.
  • Wang, Y., Harmon, N.J., Sahin-Tiras, K., Wohlgenannt, M. and Flatté, M.E., 2014. Anomalous organic magnetoresistance from competing carrier-spin-dependent interactions with localized electronic and nuclear spins. Physical Review B, 90(6), p.060204.
  • Yang, S.H., Le Rendu, P., Nguyen, T.P. and Hsu, C.S., 2007. Fabrication of MEH-PPV/SIO2 and MEH-PPV/SIO2 nanocomposites with enhanced luminescent stabilities. Reviews on Advanced Materials Science, 15(2), pp.144-149.
  • Mahmoud, F.A., Elazab, I., Abo-Elenien, O.M., Abdel Fatah, A. and Ahmed, A.A., 2019. Optical characterization of Poly [2-methoxy-5-(2-ethylhexyloxy-p-phenylene vinylene](MEH-PPV): C60, MEH-PPV: C60: TiO2 and MEHPPV: C60: ZnO Thin Films. Egyptian Journal of Chemistry, 62(2), pp.311-323.
  • Zang, H., Xu, Z. and Hu, B., 2010. Magneto-optical investigations on the formation and dissociation of intermolecular charge-transfer complexes at donor− acceptor interfaces in bulk-heterojunction organic solar cells. The Journal of Physical Chemistry B, 114(17), pp.5704-5709.
  • Shakya, P., Desai, P., Kreouzis, T., Gillin, W.P., Tuladhar, S.M., Ballantyne, A.M. and Nelson, J., 2008. The effect of applied magnetic field on photocurrent generation in poly-3-hexylthiophene:[6, 6]-phenyl C61-butyric acid methyl ester photovoltaic devices. Journal of Physics: Condensed Matter, 20(45), p.452203.
  • Lei, Y., Song, Q., Zhang, Y., Chen, P., Liu, R., Zhang, Q. and Xiong, Z., 2009. Magnetoconductance of polymer–fullerene bulk heterojunction solar cells. Organic electronics, 10(7), pp.1288-1292.
Toplam 32 adet kaynakça vardır.

Ayrıntılar

Birincil Dil İngilizce
Konular Yoğun Maddenin Elektronik ve Manyetik Özellikleri; Süperiletkenlik, Yoğun Madde Fiziği (Diğer)
Bölüm Makaleler
Yazarlar

Kevser Şahin Tıraş

Proje Numarası FBA- 2022-11983
Erken Görünüm Tarihi 30 Nisan 2024
Yayımlanma Tarihi 30 Nisan 2024
Gönderilme Tarihi 5 Mart 2024
Kabul Tarihi 19 Mart 2024
Yayımlandığı Sayı Yıl 2024 Cilt: 40 Sayı: 1

Kaynak Göster

APA Şahin Tıraş, K. (2024). Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi, 40(1), 68-74.
AMA Şahin Tıraş K. Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi. Nisan 2024;40(1):68-74.
Chicago Şahin Tıraş, Kevser. “Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping”. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi 40, sy. 1 (Nisan 2024): 68-74.
EndNote Şahin Tıraş K (01 Nisan 2024) Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi 40 1 68–74.
IEEE K. Şahin Tıraş, “Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping”, Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi, c. 40, sy. 1, ss. 68–74, 2024.
ISNAD Şahin Tıraş, Kevser. “Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping”. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi 40/1 (Nisan 2024), 68-74.
JAMA Şahin Tıraş K. Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi. 2024;40:68–74.
MLA Şahin Tıraş, Kevser. “Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping”. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi, c. 40, sy. 1, 2024, ss. 68-74.
Vancouver Şahin Tıraş K. Efficiency Improvement of Organic Photovoltaic Solar Cells via Spin Radical Doping. Erciyes Üniversitesi Fen Bilimleri Enstitüsü Fen Bilimleri Dergisi. 2024;40(1):68-74.

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